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Home > About the Academy > Biographical memoirs
BIOGRAPHICAL MEMOIRS
John Maxwell Cowley 19232004
By A. F. Moodie and J. C. H. Spence
This memoir was originally published in Historical Records of Australian Science, vol.17, no.2, 2006.
Numbers in brackets refer to the bibliography at the end of the text. The first number refers to the bibliography section, the second to the item number within that section.
John Cowley contributed significantly to all of the fields
that relate to electron diffraction and electron microscopy, and helped to
found not a few of them. His name is associated in particular with n-beam
dynamical theory, high-resolution electron microscopy, scanning transmission
electron microscopy, instrumental design, and the application of the techniques
of electron scattering to structure analysis. His experimental work was not,
however, confined to the scattering of electrons: to take but one instance, his
seminal work on the theory of short-range order was stimulated initially by his
experiments using X-rays, and it was only later that he extended the technique
to include electron diffraction. Finally, to all those who practise the
techniques of scattering electrons, X-rays, or neutrons in the study of solids,
liquids or gases, his book Diffraction Physics remains not only
eminently readable but authoritative.
With the death of John
Cowley the worlds of crystallography, microscopy and materials lost a great
scientist, those who knew him personally lost a friend, and those of us who had
the privilege of working with him lost, in addition, a mentor. For working with
John was a remarkable experience. His insight into the fundamental physics
underlying some, frequently confused, phenomenon was eerie and allowed him to
describe and then analyse the situation in often deceptively simple but in
fact decisive mathematical language.
Under those circumstances it
might very well be imagined that collaboration with John would only have been
possible for those few with commensurate abilities. As many of us can testify,
however, this was not the case, for John was possessed not only with a gift for
exposition, but also with the patience to impart what frequently must have
seemed obvious to him, in an enlightening rather than in a demoralizing way.
Few have not experienced the illusion unwittingly created by a brilliant
speaker that an intricate subject has now become transparent, but the insights
that John imparted proved permanent. How this was achieved is far from clear,
but an important contributing factor must have been his extraordinary ability
to relate key steps in a process to experimentally realisable situations, a
facility he possessed from very early in his career. Nor were the experiments
that he invoked a theorist's abstractions for, like so many of the great
crystallographers, he was equally at home at the bench, at the desk and,
indeed, as a designer in the workshop.
John's abilities were
appreciated by his family early in his life. His forebears, mostly wheat and
sheep farmers, settled in South Australia in 1845, and the tradition of country
living persisted into his parents' generation. As a consequence, John's early
education was pursued in a succession of small country state schools as his
father, a Methodist minister, was called to a succession of circuits. His
parents were determined that their four children should enjoy the educational
opportunities that circumstances had denied them, and in this they succeeded
handsomely with three graduating from the University of Adelaide. John started
his secondary education in a country state school but almost immediately won a
scholarship to Prince Alfred College, where, in turn, he won the scholarship
that took him to the University of Adelaide in 1940 at the age of seventeen.
He obtained a first class honours in physics in 1943 and an MSc in 1945. At
that time, while the physics department had few staff and limited resources, it
enjoyed a well-deserved reputation in the training of its students. In
particular, both John and an earlier student, Sir Mark Oliphant, both
acknowledged that they benefited greatly from the guidance of the Senior
Lecturer, Dr R. S. Burdon.
It was in those years that
John first encountered electron diffraction and came into direct contact with
wave-particle duality. While he was always mindful of Bohr's assessment of
those who believed that they understood quantum mechanics, John never appeared
to have any doubt as to how he might set about describing a quantum system,
relishing and by no means being dismayed by anti-intuitive outcomes. As many of
his colleagues can attest, the wave nature of the electron was no remote or
discouragingly abstract conception to him. Peering at the viewing screen while
he manipulated the controls of an electron microscope, he could be seen to be
thinking in terms of wave functions.
His work in Adelaide brought
him to the attention of Dr Ian (later Sir Ian) Wark, Chief of the Division of
Industrial Chemistry of Australia's Council for Scientific and Industrial
Research (CSIR, later CSIRO); and of Dr Lloyd Rees, who encouraged him to join
the Chemical Physics Section, just then being set up in the Division under
Rees' leadership. The broad intention behind the formation of this Section was
to ensure that expertise in emerging techniques in physics that were likely to
find application in chemistry should be available within CSIR. In addition,
Lloyd Rees laid a particular emphasis on the development of novel instruments.
Since staff were expected to
combine long-term research with collaborative work on short-term projects of
immediate application, both Wark and Rees devoted a good deal of consideration
to the selection of those who might be supposed to possess both the ability and
the temperament appropriate to such varied activities. John Cowley fitted
happily into this category and his impact was immediate. Within the next three
years he had designed and brought into operation an X-ray diffractometer,
collaborated in the design and operation of a high-resolution electron diffraction
camera (1,18)* and, along with a number
of colleagues, published papers on subjects ranging from the structure of
industrially significant minerals (1,5), through aspects of yielding in steel
(1,3) to lubrication (1,7), solid-state rectifiers (1,8) and the refraction of
electrons in polyhedral crystals (1,2).
To undertake the design of a
high- resolution electron diffraction camera in many ways typified John's
outlook. It was the conventional wisdom of the time that nothing significant
remained to be resolved, but John, while giving due weight to tradition, never
allowed himself to be dominated by it. In this he was in entire agreement with
his section leader, Lloyd Rees, and, though neither knew it at the time, with a
brilliant young Japanese theorist, Norio Kato.
At this juncture John was
granted leave of absence to study for a PhD under the direction of Professor R.
Warren at Massachusetts Institute of Technology in the United States; and it
was here that, arguably, he first attracted wide international attention with
his work, both experimental (1,9) and theoretical (1,10), on order in alloys.
This was a subject that he had not previously encountered but, starting from
the BraggWilliams foundations, a penetrating analysis led him to a
quantitative description that has proved to be of central importance to the
entire subject. Few metallurgists would fail to recognise the patterns deriving
from the memorable analysis of Cu3Au. Indeed these patterns have an
aesthetic as well as a scientific appeal. They have been incorporated in the
decoration of fabrics and, memorably, form the dust jacket of Professor
Warren's Festschrift.
On his return to Melbourne, John again became involved in a variety of what might seem to be unusually
diverse projects. To appreciate the reasons for this, it is relevant to recall
something of the policy obtaining in CSIRO at that period. The organization
addressed problems and opportunities, industrial, agricultural and social, of
relevance to Australia. This was interpreted, as it proved with great success,
by Lloyd Rees as inclusive of approaches that might range from routine
competence in, say, analysis, to the devising of completely novel techniques.
John was adept and enthusiastic in work of direct application as well as in the
wider fields with which he is usually associated and he was, accordingly, in
great demand as a collaborator in, for instance, mineralogy, metallurgy and
catalytic, inorganic and clay chemistry.
Two main themes emerged,
however, in his longer-term work, namely the extraction of structural
information from single- crystal electron diffraction patterns (1,13) and the
quantitative analysis of dynamical scattering data. The motivation for both
those lines of inquiry derived from the desire to extract structural, as
distinct from merely geometric, information from electron diffraction
patterns. In particular, John's intention was to exploit advantages deriving
from either electron optics or scattering processes peculiar to electrons.
In addressing
structure-analytical problems in electron diffraction at this juncture, John
was continually mindful of the limitations imposed by the first Born approximation
and what later became known as the phase-grating approximation, but within
those limitations he not only established a framework for analysis, he
illustrated his approach by the determination of a wide variety of structures.
This work exemplifies equally his powerful grasp of structure-analytical
technique, of the niceties of electron interaction, and of orderdisorder
phenomena. The investigation into various structural aspects of boric acid
constitutes a particularly striking example (1,15).
A very different but equally
influential example is the work undertaken with Professor J. Ibers, a
colleague from America, and Dr Robert Croft, a chemist from within CSIRO, on
the determination of the structure of that prototypic intercalate, ferric
chloride-graphite (1,25). Here the advantages to be gained, relative to X-ray
diffraction, stemmed largely from the inherently limited order in the compound.
Electron optics could be employed to illuminate a relatively small area so
that quasi- single-crystal patterns could be obtained, and since the order in
the direction of the beam was also limited, dynamical effects were such that,
with discretion, structural information could be successfully extracted. The
word discretion is important here, for in this type of work, John did not
establish prescriptions; rather he demonstrated what was possible, and
moreover possible for a range of materials not accessible to conventional
approaches.
The second theme is best
represented by his collaborative work with Peter Goodman and Lloyd Rees on
dynamical fine structure (1,27). Here, contact was made with the theoretical
work of Norio Kato who, without using the column approximation, predicted the
nature of dynamical fine structure from a wedge, using Bethe's formulation in
the two-beam approximation. Kato, who had been assured that the patterns that
he predicted could never be observed, always regarded the utilization of his
theoretical predictions in the subsequent publication in Acta Crystallographica
as a turning point in his career. Resolution of the dynamical fine structure stemmed directly
from the insight shared by Lloyd and John in assessing the need for high
angular resolution in electron diffraction, and in their skill in achieving it.
Dynamical theory at this juncture had become virtually synonymous with the
two-beam approximation introduced by Ewald in his dynamical theory of X-ray
scattering, and by Bethe in his dynamical theory of electron diffraction. This
was far from the initial intention of either of these men but a variety of
historical misconceptions, deriving largely from experimental deficiencies,
led many to this view. However, any direct extension to many beams certainly
raised formidable difficulties.
The opportunity to initiate an
oblique approach arose as a result of a chance observation of a distant sodium
street light in the Melbourne suburb of Oakleigh, when observed through a nylon
kitchen curtain of rather precise weave. This raised questions about the
imaging of periodic objects (1,28), questions that had scarcely been examined
since Lord Rayleigh won a medal presented by the Royal Society for a
description of scattering from a simple one-dimensional acoustic grating. (The
calculation was undertaken in response to a question raised by Fox Talbot on
the origin of the difficulty in obtaining precise focus on an optical grating.)
In order to describe in
compact form, say, the scattering of light by a general two- dimensional phase
grating illuminated by a source of finite size, it was found convenient,
working in the paraxial approximation, to rewrite the standard equations in a
form where the techniques of the Fourier transform could be readily exploited
(1,32). The multiple focal planes that were found to be generated in fact,
the planes of the Fourier images could then be assessed in relation to the
electron microscopy of crystals at atomic resolution. This development, in
turn, raised in acute form the need for an explicit solution to the problem of
the scattering of electrons by a crystal into an arbitrary number of beams.
The technique that had been
found effective in the description of scattering from periodic objects was
therefore generalized so that scattering by a sequence of objects was
described in co-ordinate space by alternating multiplication by transmission
functions with convolution by Fresnel propagators. A crystal is then envisaged
as being cut into parallel slices of arbitrary thicknesses, not necessarily
equal. The contents of the slices are projected on to planes that act as
two-dimensional mixed phase and amplitude gratings to modulate the wave
function, which, in turn, propagates between the planes.
In practice it was found
convenient to work in momentum space, where the operators for multiplication
and convolution are interchanged and act on the Fourier transforms of the
transmission functions and the propagators. Symmetries inherent in the
propagators greatly simplify the calculations. The calculation is then carried
through and the impulse limit taken; that is, the number of slices is taken to
infinity as the thicknesses of the slices go to zero, in such a way that the
product of number and thickness remains finite and equal to the thickness of
the crystal. An explicit solution is obtained in the form of an infinite series
in ascending order of interaction (1,31) in effect, a Born series. In
retrospect, various transformed versions of the solution seem almost obvious,1
but various delicate mathematical points are involved in the limiting process
and these were not explored in the initial submission. A good deal later it was
shown that this 'multislice' method, as it became known, is closely related to
that of Feynman quantum mechanics, that the problems in measure are equivalent
and by no means trivial, but that the procedure ultimately leads to the
Schrφdinger equation.2 It was not, in the event, for reasons
related to measure that John's manuscript was initially rejected, but
basically because of misconceptions over the role of eigenvalues and
eigenvectors in quantum mechanics. Intervention by one of the originators of
dynamical theories reversed the decision, however, and the paper was published
unchanged.
Within a few
years the same solution had been obtained by other techniques, all of which
could be shown to be equivalent (1,43). The solution that emerged, in its many
and varied forms, along with its theoretical, experimental and numerical
ramifications, still occupies many in the disciplines of electron diffraction
and in the equally diverse field of electron microscopy.
At this juncture, a
development that was to extend over the years began to emerge, with
collaborators in significant numbers and from all quarters of the world gathering
round John. His high abilities as a teacher became increasingly apparent, and
his accession to the Chamber of Manufactures Chair of Physics in the University of Melbourne in 1962 seemed not only appropriate but virtually inevitable. Here
he set up a highly individual school of extraordinary productivity, numbering
amongst its graduates some of the most distinguished current workers in the
field. During this period he also wrote Diffraction Physics
(4,1), one of the central texts in crystallography and one that has remained
indispensable, equally to two generations of students and to their
supervisors. In its directness, clarity and simplicity it bears, as all great
scientific books do, an unmistakable personal stamp.
The work carried through on
many- beam scattering had treated inelastic interactions by assigning an
absorption coefficient to each structure amplitude. This is limited to
providing only phenomenological descriptions of, say, Borrman effects. John
set about repairing this deficiency and, in a series of papers (1,52) with his
post-graduate students, laid the foundations for what has evolved into a field
in its own right, extending into microscopy as well as diffraction.
The
development of n-beam theory had been stimulated equally by diffraction and
microscopy and central points having been established in diffraction,
applications could be confidently undertaken in microscopy. The resolution now
available in commercial electron microscopes was just sufficient to explore
crucial points raised by Wadsley's seminal work in inorganic chemistry and
X-ray diffraction.3,4 This work had been carried through in CSIRO
and it was again in this organization that central results for instance,
confirmation of the existence of Wadsley defects and the coexistence of a
range of phases in the block oxides was established by electron microscopy,
necessarily utilizing many beams.5,6 The Wadsley defect constitutes
a delicate test since typically there is only a change in stoichiometry, with
little or no attendant strain across the 'shear plane' with vertex sharing
changing into edge sharing, say, so that near-atomic resolution is required,
even for detection. John, in part through his students,7
collaborated at an early stage in the research and this extended to incisive
work undertaken later in America on high-resolution lattice imaging, initially
of the block oxides. It was characteristic of John that his entire attention,
on this as on other occasions, was directed towards the scientific outcomes of
the inquiry. Collaboration, as ever, was therefore very straightforward. The
all too familiar difficulties involving personalities and, above all,
institutions, simply never arose.
Concurrently with these
activities, John revisited his seminal work on short-range ordering and, along
with his collaborators, substantially extended its range of application. This,
among other matters, led to the development of a graphic model involving the
curvature of the Fermi surface and its relation to the diffuse scattering
observed in the electron diffraction patterns of certain groups of materials
(1,63).
From the time of von Laue,
reciprocity, a subtle symmetry which, as it later emerged, is associated at a
fundamental level with wave equations, has at various times occupied a great
variety of crystallographers. John emphasised the importance of this symmetry
to his students, two of whom, in a key paper, invoked Green functions to
establish that reciprocity is inherent in Schrφdinger's equation and applies to
n-beam, not merely to two- beam, diffraction.8
John had always been
particularly adept at exploiting this symmetry, a notable example being
afforded by a particularly important, apparently simple and certainly short
paper that he published in 1969. This generalized previous results and, in a
stroke, revealed the relationship between images generated by transmission
electron microscopy and those generated by scanning transmission microscopy, a
matter much canvassed at that time (1,59).
The paper has an added
significance in that it reveals the direction in which John's approach to
research was turning, namely towards the development and utilization of a
highly individual, generalized scanning instrument. In designing this
instrument, John's formidable array of varied abilities were deployed in
profusion; from workshop practice through solid state physics to light and
electron optics, and to the mathematical physics of vibration and of quantum
mechanics. These efforts laid the foundations for some of the seminal work that
lay in the future.
At a
conference on solid state chemistry in Scottsdale, Arizona in 1969, Cowley was
approached by Professor Leroy Eyring about the possibility of establishing an
electron microscopy group in the Center for Solid State Science at Arizona
State University (ASU) in Tempe, near Phoenix in the United States. Cowley
moved in 1970 to take up the Galvin Chair of Physics at ASU, taking with him
from Australia his colleague Professor A. Strojnik, a mechanical workshop
instrumentation specialist, four PhD students and several postdoctoral
associates. Five other Melbourne physics PhD students also visited for shorter
periods. Supported by ASU funding and an Area Development Award from the
National Science Foundation, Cowley immediately appointed Dr S. Iijima as
his postdoctoral assistant, purchased new electron microscopes, and rapidly
established one of the leading international groups in electron microscopy and
diffraction physics. John Spence, who completed his PhD in physics at Melbourne under Allan Spargo during Cowley's time there, was to join the group as a
faculty member in 1977 following postdoctoral work in Oxford. In 1971, Cowley
took on the co-editorship of Acta Crystallographica for about a
decade and the directorship of the Electron Microscopy Society of America from
1971 to 1974. He served as the International Union of Crystallography's
representative on the Commission for Solid State Physics from 1969 to 1978.
In 1970, more
than ten years after Menter's first lattice images, the resolution of the best
high-resolution electron microscope (HREM) images was about 0.34 nm. In Chicago, Albert Crewe had just demonstrated that individual, well-separated heavy atoms
could be imaged using a scanning transmission electron microscope (STEM), with
the aim of applying the method to biology. (Cowley's reciprocity paper
mentioned above had established the intimate connection between STEM and HREM,
using Helmholtz's reciprocity theorem.) Cowley in 1959 had written perhaps the
first paper to analyse the effect of multiple scattering on simple lattice
images such as Menter's, using two-beam theory. In Australia, the CSIRO group
led by A. Moodie had begun to demonstrate the usefulness of HREM for the
observation of planar defects in oxide crystals, in which entire planes of
atoms were missing, and to develop the appropriate imaging theory with full
allowance for multiple scattering (dynamical) effects. Dr M. O'Keefe, who had
previously worked with the CSIRO group, had also moved to ASU and was closely
involved in the early HREM projects at ASU with Cowley and Iijima. Cowley was
convinced that by improving the resolution of the microscopes to the atomic
level for the much smaller spacings present in crystals, a large scientific
payoff could be obtained in the solid state sciences. His view was that since
most of the electronic, thermal, mechanical and magnetic properties of
condensed matter for example in first-order phase transitions, plasticity and
non-stoichiometry are controlled by defects such as atoms missing from the
periodic arrangement of a crystal, it followed that HREM was the ideal tool for
their study, and the challenge was to improve image resolution accordingly. He
was one of the first to appreciate the full power of HREM in materials science,
solid state chemistry and condensed matter physics, and he devoted
extraordinarily energetic efforts to its development over several decades.
By taking advantage of a
specially modified pole-piece fitted to a Japanese electron microscope,
Iijima and Cowley were able to publish a series of papers in the early 1970s
that both laid down the theoretical principles for high-resolution imaging of
thin crystals in various modes, and applied this theory to Iijima's remarkable
experimental images of defects in crystals.9 At that time,
following earlier work in the late 1960s by Wadsley, Moodie, Bursill, Allpress,
Sanders and co-workers at slightly lower resolution, it was realised that
non-stoichiometry in complex oxides could be accommodated by planar faults.
Non-stoichiometry refers to local deviations in the ratio of the amounts of
the various types of atoms present in a crystal, usually taken to be constant
for a given chemical formula. Planar faults, in addition to the point defects
previously assumed, were discovered. These point defects may consist of
individual missing atoms or groups of atoms. This finding had important
implications for thermodynamics, for our understanding of the structural
relationships between oxides, and for the mechanisms of oxygen uptake in
minerals and catalysts. The instruments of that time provided 'unit-cell'
resolution, so that the arrangement of the fundamental building blocks of many
transition metal oxides could be determined in projection by high-resolution
electron microscopy. Iijima and Cowley published the first clear
two-dimensional image of Wadsley's defect (1,64), giving confidence in the
earlier theoretical and experimental work of the Australian groups on the type
of mistakes that can occur in the periodic arrangement of atoms in these
crystals. This analysis of planar faults in oxides expanded rapidly in the
hands of many experts around the world, and has continued since. Its origins
at CSIRO and later ASU represent probably the first occasions on which
scientifically significant high- resolution information had been extracted at
the near-atomic scale from crystals by the new method of HREM 'lattice imaging'.
Disorder of various kinds in oxides remained a theme in all Cowley's HREM work,
including the classic study with Yagi using combined HREM images and point
diffraction patterns of potassium ion ordering in KSbO3 in 1978
(1,91), which is typical of this interest of Cowley's. It shows Cowley's
natural flair for the interpretation of diffuse scattering (which is a
continuous function of scattering angle, rather than the sharp Bragg peaks
normally generated by crystals) in terms of ordering in real space, and of the
effects of multiple scattering on it. Following publication of a major review
article on electron diffraction for structure analysis (1,56), it is clear that
in these years Cowley's main interest had turned to imaging in all modes transmission, reflection and scanning. He was to return to diffraction in
new and imaginative ways in the 1980s, in the development of the
nanodiffraction method.
In a
remarkable burst of energy, with generous support from ASU, the National
Science Foundation and other agencies, Cowley took on a large number of
students at ASU and established new instrumentation and theory projects in
several areas. At one point his group numbered more than a dozen PhD students.
With A. Strojnik (and later D. Smith, another Melbourne graduate arriving from
a post-doc at Cambridge), a 1-MeV STEM was constructed at ASU, intended for
imaging thicker inorganic samples and, amongst other things, to allow
high-resolution imaging of biological samples in air. (These were to be
attached to a thin carbon membrane that formed the vacuum seal at the electron
beam focus.) In other work in biology, Cowley had in 1971 (1,61) investigated
the assumption of absorption contrast (rather than phase contrast), and the
neglect of multiple scattering, in the tomographic transmission electron micoscopy
work then just starting in Cambridge and elsewhere. Cowley's monograph Diffraction Physics, which first appeared in 1975 (4,1), is now in its third
edition, and set the agenda for much of the physics of electron microscopy
that was to follow. The book, which treats electron, X-ray and neutron diffraction,
covers his main interests up to that time the theory of multiple elastic and
inelastic scattering, scattering from defects in crystals, HREM and STEM
imaging, and the statistical mechanics of ordering in alloys. A second major
novel instrumentation project started in the early 1970s with G. Hembree and
others consisted of a field- emission reflection high energy electron
diffraction (RHEED) system that produced scanning reflection images and micro-diffraction
patterns from atomically clean surfaces (1,152). This pioneering work occurred
in the very early days of the field- emission electron source.
Just as
mistakes in atomic positioning and species within otherwise periodic
crystallline material may control its bulk properties, irregularities on the
surfaces of crystals control the chemical interactions of crystals with their
environment. This can be crtically important in areas of science as diverse as
catalysis and corrosion. Yet prior to 1980 there were no methods that provided
atomic-resolution images of extended crystalline surfaces. Cowley saw clearly,
a decade before the invention of the scanning tunnelling microscope, the
potential power of a high- resolution imaging method in surface science, to
complement the then-popular broad-beam Low Energy Electron Diffraction (LEED)
and RHEED methods. He understood at an early stage how the difficult
interpretation of LEED patterns might be assisted by a method that combined
imaging and diffraction. With his student A. Moon, Cowley published a new
theoretical approach to dynamical RHEED theory at about this time (1,65).
Papers on the theory of RHEED for defective surfaces followed, a topic in
which he remained interested for the rest of his life, and was to return to in
his application (with L. M. Peng) of the multi-slice approach to the reflection
geometry (1,167). This in turn supported experimental work on the Reflection
Electron Microscopy (REM) imaging technique, which he developed rapidly from
its earlier primitive form. Here an image is formed from a Bragg electron beam
reflected at a low angle from a crystalline surface. In a series of papers, he
established a dynamical (multiple-scattering) theory of REM imaging for
defective surfaces, while his PhD students produced many of the most striking
images of crystal surfaces using this method (1,167). Cleaved oxides and
semiconductors and facetted gold spheres were studied, amongst other materials,
at a resolution of about one nanometer. These images showed the predicted
surface defects,
including surface steps, in some cases terminating at emerging dislocations.
The effects of image foreshortening, of elastic energy filtering, and of
dynamic focusing were all investigated, while his elegant treatment (with L. M.
Peng and P. Liu) of diffraction at a surface step has since been
widely adopted (1,190). His own experimental work at this time produced the
scanning reflection electron microscopy (SREM) method, which is conveniently
combined with reflection microdiffraction analysis (1,136; 1,257). Using this,
by combining reflection microdiffraction patterns from nanometer-sized areas
with the corresponding scanning images, he was able to explain many of the
diffuse scattering effects seen in RHEED (1,226), and to distinguish, for
example, streaking due to surface steps from that due to inelastic scattering.
This work led to studies on the surface resonance effect with his students Z.
L. Wang, L. M. Peng and others (1,214). His earliest work on REM began during a
visit to ASU from Professor K. Yagi in the early 1970s. Yagi and his student
Takayanagi were to use similar methods to powerful effect in Japan soon afterwards in solving the famous silicon (111) (7 Χ 7) reconstruction,
often described at that time as the last great problem in surface
crystallography.
Cowley's early paper on
STEM/TEM reciprocity kindled an enthusiasm for the STEM mode that remained to
the end of his life. (In simplest form, this reciprocity theorem allows
ray-paths to be reversed in an optical system, suggesting interesting new
scientific instrument designs and signals to be detected.) During the 1970s,
Cowley also produced a series of papers on novel imaging modes in STEM (1,88),
culminating in the arrival in 1978 of a Vacuum Generators HB-5 STEM electron
microscope, funded by his National Science Foundation grant, that he personally
operated from that time until the last week of his life. Cowley designed an
ingenious optical-image dissection device that converted electron nanodiffraction
patterns produced by a vacuum-coupled image intensifier to optical images, portions
of which could be led off to various detectors, with a flexible masking system
(3,27). A typical project (with G. Butler, M. Strahm and later G. Fan, from
1980) using this system involved the automated collection of many coherent
microdiffraction patterns from nanometer-sized areas of thin glassy films, in
order to characterize their structure. For the problem of short and medium
range order in glasses, Cowley was convinced of the value of nanodiffaction for
the extraction of information on angular correlations between bond angles, thus
going beyond the limitations of the radial distribution function commonly used
(3,27). In other work at this time with Spence, the theory of atomic resolution
imaging by STEM in thin crystals was elaborated (1,93), emphasising the role
of interference between overlapping coherent covergent-beam electron
diffraction (CBED) orders, an effect previously detected by Dowell and Goodman.10
This dynamical 'ptychography' (from the Greek 'to fold') results when a cone
of illuminating rays is used so large that the Bragg diffraction orders overlap
and interfere. The analysis of coherent nanodiffraction patterns from thin
crystals (1,104) soon led also to his work on in-line electron holography, from
which he developed an elegantly simple relationship between in-line holograms
in STEM, shadow images and the Talbot self- imaging properties of thin crystals
(1,250). This work in turn led to the development of the theory of electron
Ronchigrams in the early 1980s (1,165). These electron interferograms, similar
to those used to characterize astronomical optical elements, have become the
standard method of automated alignment and aberration measurement in modern
aberration-corrected magnetic lenses. The recent attainment of sub-Εngstrom-resolution STEM
imaging depends heavily on Cowley's development and analysis of these patterns.
The early 1980s were an
exciting time for the ASU group, with the influx of several new faculty
appointments and outstanding postdoctoral researchers in Cowley's field.
These appointments by a supportive ASU administration followed the National
Science Foundation's award in 1979 of about $US1,500,000 (for three years) for
a continuing grant for a regional and later national instrumentation facility
for high-resolution electron microscopy at ASU, directed by Cowley. Ondrej
Krivanek, David Smith, Ray Carpenter and Peter Rez, as new appointments, worked
with existing professors Leroy Eyring, Peter Buseck and John Spence, and later
John Venables, on lively management meetings of 'the facility', in which many
new scientific projects were devised and funded. These spanned the scientific
interests of the faculty, from the earth sciences to solid state physics and
chemistry and surface science. Additional supportive appointments for
tenure-track full-time researchers made in the Center for Solid State Science
included G. Hembree and later M. Scheinfein. Postdocs included J. Tafto,
Y. Bando, N. Long, D. Shindo and D. Veblen, amongst many others. The mission of
the facility, the development and application of HREM, required an extensive
user programme, an annual international conference ('workshop'), and a winter
school each year to teach the practical methods of HREM. Cowley took on this
considerable workload with the support of the management committee and
particularly that of the laboratory manager John Wheatley and his assistants,
who were responsible for the upkeep of the transmission electron microscopes of
various types, eventually eight in number. The dedication of the four technical
staff of the facility was crucial to its success, which saw a continuous stream
of national and international visitors and microscope users that has continued
ever since. The idea was to teach the methods of HREM to scientists in
universities, national laboratories and companies in the USA and elsewhere, to develop new related techniques, and to apply them to all areas of
solid state and surface science. The ambitious aim was to explain the
properties of matter in terms of the atomic structures and processes seen in
the electron microscopes, by combining these experimental results with a
vigorous programme of theoretical analysis. This was Cowley's bold vision
during the 1980s, during which the resolution of the transmission electron
microscopy instruments improved from about 0.26 to 1.4 nm. In most cases this
was not quite sufficient to resolve individual columns of atoms in projection,
so that a considerable theoretical effort was devoted to image interpretation.
Unlike other groups, Cowley's approach included all multiple scattering effects
from the beginning. Following Iijima's return to Japan, David Smith in later
years took on the job of running the schools and workshops. Following Cowley's
death in May 2004, the facility has been re-named the J. M. Cowley Center for Electron Microscopy and is directed by Smith.
Cowley fostered a vigorous
programme of instrumentation development early versions of what
would later become the commercial Gatan electron energy loss spectrometer, and
an electronic imaging system also taken up by Gatan, were developed by
Krivenek and Spence, respectively, at that time. Much more ambitious projects,
later in the 1980s, included a special ultra-high-vacuum version of the Vacuum
Generators field-emission STEM instrument (1,227) dedicated to imaging and
anlaysis of surfaces, and an ultra-high- voltage transmission electron
microscope developed with the Gatan company. The design and development of
these two novel instruments involved much detailed collaboration between company and
ASU researchers (especially Cowley, Venables, Long, Hembree and Krivanek). The
Auger imaging system on the Vacuum Generators, for example, developed by
Venables and co-workers and based on a novel magnetic extraction field that
collected Auger electrons generated by the sub-nanometer probe over a very
large solid angle, subsequently produced record-breaking 1-nm resolution Auger
images.
The annual workshops, first
held in the Arizona desert at Castle Hot Springs and later at Wickenburg, were
memorable events. It was a remarkable achievement of Cowley's to attract to the
Arizona desert, each winter for well over a decade, leading scientists from
all around the world in fields other than electron microscopy for a small,
specialized workshop. The workshops, which quickly gained a reputation for
scientific excitement and high quality, covered some aspect of condensed matter
science to which it was thought that electron microscopy could contribute,
with papers subsequently collected together and published in the journal Ultramicroscopy.
Topics covered a wide range, from metal clusters to the imaging of clean
surfaces, solid state chemistry, diffraction and channelling methods,
interfaces, ceramics, semiconductors, mineralogy and catalysts.
The arrival of several groups
of first- rate Chinese PhD students under the ChinaUnited States Postgraduate
Exchange Agreement programme in the mid-1980s had a stimulating effect on the
group comparable only to the original influx of Australian students fifteen
years earlier. Projects included theory and practice of REM and SREM imaging
(with T. Hsu, N. Yao and L. M. Peng), and energy- loss spectroscopy in the
reflection mode (with Z. L. Wang), and work on REM and SREM imaging of steps
(1,214). In the STEM, Cowley also embarked on an analysis of planar faults by
coherent microdiffraction in the transmission geometry with Zhu and Pan
(1,135). The method was applied to antiphase domains in copper- gold alloys and
to platelets in diamond, and was later extended to the faulting found in small
metal particles and catalysts. Cowley's interest in modulated, intergrowth and
incommensurate structures continued in work with N. Tanaka, culminating in his
organization of an international conference on this topic in Hawaii and a
subsequent Gordon conference.
The publication by Pennycook
and Boatner in 1988 of high-resolution STEM images using high-angle scattering,
as proposed by Howie, led to a burst of activity at ASU and Cornell, in which
the effects of temperature and other effects on the thermal diffuse and Bragg
scattering used to form these images was investigated by Cowley, Liu, Wang and
others (1,231). The final years of Cowley's career were devoted to
microdiffraction studies of individual nanotubes (1,322), to work on ferroelectrics,
to an idea he and Smirnov had of using strings of atoms as electron lenses
(1,305), and to work with M. Scheinfein and M. Mankos on electron holography of
magnetic materials (1,283). His last project returned him to his early interest
in the structure of ferritin (1,331). Cowley became convinced from
nanodiffraction evidence that the conventionally accepted form of the iron
oxide core in ferritin was incorrect, and he proposed mechanisms for oxygen
uptake based on his novel structure, relevant to Alzheimer's disease. His
belief in the unique power of coherent electron nanodiffraction for the study
of various forms of disorder in crystals and glasses, and his ability to record
and interpret these patterns in terms of correlations amongst atom positions,
remained to the end (1,324).
Cowley received many honors
during his lifetime. These included the Edgeworth David Medal, the Research
Medal of the Royal Society of Victoria, the Warren Award of the American
Crystallographic Association (with S. Iijima),
the Distinguished Scientist Award of the Microscopy Society of America and the Ewald Prize (with A. Moodie) of the International Union of Crystallography. He was a
Fellow of the American Physical Society, of the Royal Society of Victoria, and
of the Institute of Physics, and a member of the US National Committee for
Crystallography. He was elected a Fellow of the Australian Academy of Science in 1961 and of the Royal Society of London in 1979.
John's life was almost
entirely devoted to his family and his work, and to the extensive international
travel it involved during which, in China, Japan, Europe or Australia, he would frequently encounter the extended family of his many devoted
ex-students. Apart from classical music, his main hobby was painting in oils; a
display of his fine work was mounted at a memorial meeting held in his honour
at ASU in mid-2004, attended by his daughters. Throughout his career in Melbourne and Arizona, John Cowley's calm confidence, scientific vision and sustained
industry were an inspiration to those about him. John continued experimental
work to the last day of his life. A visit to his office always left the visitor
stimulated with new ideas and inspiration always encouraging, he had a
characteristic ability to take a student's imperfectly formed ideas and to turn
them towards new and exciting possibilities with his familiar manipulations
and facility in analysis. The intimate relationship between experiment and his
intuitive theoretical insight, combined with his unflappable manner, his
generosity with ideas and support for others, and his unflagging conviction
that electron scattering and imaging were the most powerful tools for
understanding atomic processes in solids these were the characteristics that
have left so many of his colleagues in his debt. He is survived by his
daughters Jillian and Deborah and his devoted wife Roberta.
References
1. A.
F. Moodie, 'Reciprocity and shape functions in multiple scattering diagrams', Z. Naturforsch.
Teil A 27 (1972), 437440.
2. P. Goodman and A.
F. Moodie, 'Numerical evaluation of N-beam wave-functions in electron
scattering by the multi-slice method', Acta Cryst. A30 (1974), 280290.
3. A. D. Wadsley, Rev.
Pure Appl. Chem. 5 (1955), 165193.
4. A.
D. Wadsley and S. Andersson, in Perspectives in Structural Chemistry, Vol. 3.1, ed. J. D. Dunitz and
J. A. Ibers (New York: Wiley).
5. J.
G. Allpress, J. V. Sanders and A. D. Wadsley, 'Multiple phase formation in
binary system Nb205-W03. 6. Electron microscopic observation and evaluation of
non-periodic shear structures', Acta Cryst. B25 (1969), 1156.
6. J. G. Allpress, E.
A. Hewat, A. F. Moodie and J. V. Sanders, 'n-Beam Lattice Images. 1
Experimental and computed images from W4Nb26O77', Acta Cryst. A28
(1972), 528536.
7. E. A. Chidzey, MSc
thesis, University of Melbourne, 1970.
8. A. P. Pogany and
P.S. Turner, 'Reciprocity in electron diffraction and microscopy', Acta Cryst.
A24 (1968), 103109.
9. S. Iijima, 'High
resolution electron microscopy of crystal lattice of titanium-niobium oxide', J.
Appl. Phys. 42 (1971), 58915893.
10. W. C. T. Dowell and
P. Goodman, 'The influence of source size on CBED patterns', Optik 45
(1976), 9396.
Bibliography
1. Papers in refereed scientific journals
1. J.
M. Cowley and A. L. G. Rees, 'Refraction effects in electron diffraction', Nature
158 (1946), 550552.
2. J. M. Cowley and
A. L. G. Rees, 'Refraction effects in electron diffraction', Proc. Phys. Soc.
59 (1947), 287302.
3. J. M. Cowley and
M. S. Patterson, 'X-ray diffraction studies of yielding in mild steel', Nature
159 (1947), 846847.
4. J. M. Cowley and
T. R. Scott, 'The nature of precipitated sodium fluo-aluminates', J. Am. Chem.
Soc. 69 (1947), 25962598.
5. J. M. Cowley and
T. R. Scott, 'Basic fluorides of aluminum', J. Am. Chem. Soc. 70 (1948),
105109.
6. N. S. Bayliss, J.
M. Cowley, J. L. Farrant and G. L. Miles, 'The thermal decomposition of
synthetic and natural alunite: investigation by X-ray diffraction,
electron diffraction and electron microscope methods', Aust. J. Sci. Res.
A1 (1948), 343350.
7. J. M. Cowley,
'Electron diffraction by fatty acid layers on metal surfaces', Trans. Farad.
Soc. 44 (1948), 6068.
8. J. M. Cowley and
J. L. Symonds, 'Electron diffraction and rectification from silicon and pyrite
surfaces', Trans. Farad. Soc. 44 (1948), 5360.
9. J. M. Cowley,
'X-ray measurement of order in single crystals of Cu3Au', J.
Appl. Phys. 21 (1950), 2430.
10. J. M. Cowley, 'An
Approximate theory of order in alloys', Phys. Rev. 77 (1950), 669675.
11. J. M. Cowley, A. L.
G. Rees and J. A. Spink, 'The morphology of zinc oxide smoke particles', Proc.
Phys. Soc. 64 (1951), 638649.
12. J. M. Cowley and A.
L. G. Rees, 'Secondary elastic scattering in electron diffraction', Proc.
Phys. Soc. 64 (1951), 609619.
13. J. M. Cowley,
'Structure analysis of single crystals by electron diffraction. I. Techniques',
Acta Cryst. 6 (1953), 516522.
14. J. M. Cowley,
'Electron diffraction study of hydrogen bonds in boric acid', Nature 171
(1953), 440442.
15. J. M. Cowley,
'Structure analysis of single crystals by electron diffraction. II Disordered
boric acid structure', Acta Cryst. 6 (1953), 522529.
16. J. M. Cowley,
'Structure analysis of single crystals by electron diffraction. III. Modifications
of alumina', Acta Cryst. 6 (1953), 846853.
17. J. M. Cowley,
'Stacking faults in gamma-alumina', Acta Cryst. 6 (1953), 5354.
18. J. M. Cowley and A.
L. G. Rees, 'Design of a high-resolution electron diffraction camera', J.
Sci. Inst. 30 (1953), 3336.
19. J. M. Cowley, 'A
new microscopy principle', Proc. Phys. Soc. 66 (1953), 10961100.
20. J. M. Cowley,
'Intensity anomalies in electron diffraction patterns of CuO', J.
Electrochem. Soc. 101 (1954), 277280.
21. J. M. Cowley,
'Electron diffraction patterns of CuO', J. Appl. Phys. 27 (1956), 422.
22. J. M. Cowley, 'A
modified Patterson function', Acta Cryst. 9 (1956), 397398.
23. J. M. Cowley,
'Stereoscopic three-dimensional structure analysis', Acta Cryst. 9
(1956), 399401.
24. J. M. Cowley,
'Electron diffraction study of the structure of basic lead carbonate, 2PbCo3.Pb(OH)2',
Acta Cryst. 9 (1956), 391396.
25. J. M. Cowley and J.
A. Ibers, 'The structure of some ferric chloride-graphite compounds', Acta
Cryst. 9 (1956), 421431.
26. J. M. Cowley, 'On
order-disorder structures', Acta Cryst. 10 (1957), 141.
27. J. M. Cowley, P.
Goodman and A. L. G. Rees, 'Crystal structure analysis from fine-structure in
electron diffraction patterns', Acta Cryst. 10 (1957), 1925.
28. J. M. Cowley and A.
F. Moodie, 'Fourier images, I. The point source', Proc. Phys. Soc. B
70 (1957), 486496.
29. J. M. Cowley and A.
F. Moodie, 'Fourier images, II. The out-of-focus patterns', Proc. Phys. Soc. B 70 (1957), 497504.
30. J. M. Cowley and A.
F. Moodie, 'Fourier images, III. Finite sources', Proc. Phys.
Soc. B 70 (1957), 505513.
31. J. M. Cowley and A.
F. Moodie, 'The scattering of electrons by atoms and crystals. I. A new
theoretical approach', Acta Cryst. 10 (1957), 609619.
32. J. M. Cowley and A.
F. Moodie, 'A new formulation of scalar diffraction theory for restricted
aperture', Proc. Phys. Soc. 71 (1958), 533545.
33. J. M. Cowley and A.
F. Moodie, 'The scattering of electrons by atoms and crystals. II. The effect
of finite source size', Acta Cryst. 12 (1959), 353359.
34. J. M. Cowley and A.
F. Moodie, 'The scattering of electrons by atoms and crystals. III.
Single-crystal diffraction patterns', Acta Cryst. 12 (1959), 360367.
35. J. M. Cowley, 'The
electron-optical imaging of crystal lattices', Acta Cryst. 12 (1959),
367375.
36. J. M. Cowley and A.
F. Moodie, 'Electron diffraction and imaging effects for superimposed thin
crystals', Acta Cryst. 12 (1959), 423428.
37. J. M. Cowley,
'Short- and long-range order parameters in disordered solid solutions', Phys.
Rev. 120 (1960), 16481657.
38. J. M. Cowley and A.
F. Moodie, 'Fourier images, IV. Phase gratings', Proc. Phys. Soc. 76
(1960), 378384.
39. J. M. Cowley, A. F.
Moodie, Shizuo Miyake, Satio Takagi and Fuminori Fujimoto, 'The extinction rule
for reflections in symmetrical electron diffraction spot patterns', Acta Cryst.
14 (1961), 8788.
40. J. M. Cowley and A.
F. Moodie, 'Out-of- focus electron microscope images of edges of crystal
lattices', Nature 189 (1961), 477478.
41. J. M. Cowley,
'Diffraction intensities from bent crystals', Acta Cryst. 14 (1961),
920927.
42. J. M. Cowley and A.
Goswami, 'Electron diffraction patterns from montmorillonite', Acta Cryst.
14 (1961), 10711079.
43. J. M. Cowley and A.
F. Moodie, 'The scattering of electrons by thin crystals', J. Phys. Soc. Japan
17, Supplement B-II (1962), 8688.
44. J. M. Cowley and
Shigeya Kuwabara, 'Electron diffraction intensities from polycrystalline
materials containing heavy atoms', Acta Cryst. 15 (1962), 260270.
45. F. Aragon de la
Cruz and J. M. Cowley, 'Structure of graphitic oxide', Nature 196
(1962), 468469.
46. F. Aragon de la
Cruz and J. M. Cowley, 'An electron diffraction study of graphitic oxide', Acta
Cryst. 16 (1963), 531534.
47. J. M. Cowley,
'Electron diffraction study of evaporated beryllia', Nature 204 (1964),
1082.
48. J. M. Cowley, 'The
derivation of structural information from absorption effects in X-ray
diffraction', Acta Cryst. 17 (1964), 3340.
49. J. M. Cowley,
'Short-range order and long- range order parameters', Phys. Rev. 138
(1965), A1384A1389.
50. J. M. Cowley,
'Atomic ordering: short-range order in alloys', J. Aust. Inst. Metals 11
(1966), 258263.
51. J. M. Cowley,
'Irradiation effects in beryllia and zinc oxide', Acta Cryst. 21 (1966),
192196.
52. J. M. Cowley and A.
P. Pogany, 'Diffuse scattering in electron diffraction patterns. I. General
theory and computational methods', Acta Cryst. A24 (1968), 109116.
53. J. M. Cowley,
'Diffuse scattering in electron diffraction patterns. II. Short-range order
scattering', Acta Cryst. A24 (1968), 329-.
54. J. M. Cowley, 'The
channelling of fast charged particles through crystals', Phys. Lett. A
26 (1968), 623625.
55. J. M. Cowley,
'Kinematical diffraction from solid solutions with short-range order and size
effect', Acta Cryst. A24 (1968), 557563.
56. J. M. Cowley, 'The
determination of structure factors from dynamical effects in electron
diffraction', Acta Cryst. A25 (1969), 129134.
57. P. S. Turner and J.
M. Cowley, 'The effects of n-beam dynamical diffraction on electron diffraction
intensities from polycrystalline materials', Acta Cryst. A25 (1969),
475481.
58. J. M. Cowley,
'Electron diffraction intensities of Kossel and Kikuchi lines', Zeits. f.
angewandte Physik 26 (1969), 149154.
59. J. M. Cowley,
'Image contrast in transmission scanning electron microscope', Appl. Phys. Lett.
15 (1969), 5859.
60. J. M. Cowley and S. Kuwabara, 'Information on excited states of crystals from inelastic electron diffraction
intensities', Phys. Lett. 34A (1971), 135136.
61. G. R. Grinton and
J. M. Cowley, 'Phase and amplitude contrast in electron micrographs of
biological material', Optik 34, 221 (1971), 221233.
62. David J. Smith and
J. M. Cowley, 'Line patterns in wide-angle convergent beam electron
diffraction', J. Appl. Cryst. 4 (1971), 482487.
63. J.
R. Castles, J. M. Cowley and A. E. C. Spargo, 'Short-range ordering of
vacancies and Fermi surface of TiO', Acta Cryst. A27 (1971), 376383.
64. J. M. Cowley and
Sumio Iijima, 'Electron microscope image contrast for thin crystals', Zeit.
f. Naturforsch. 27A, 445 (1972), 445451.
65. A. R. Moon and J.
M. Cowley, 'Medium energy electron diffraction', J. Vac. Sci. Tech. 9
(1972), 649651.
66. J. R. Sellar and J.
M. Cowley, 'Resolution and contrast in high voltage scanning electron
microscopy', in 'Scanning Electron Microscopy, 1973', ed. Om Johari, IIT
Research Inst., Chicago (1973), 243250.
67. J. M. Cowley and H.
Shuman, 'Electron diffraction from a statistically rough surface', Surface
Sci. 38 (1973), 5359.
68. J. M. Cowley, 'High
resolution dark-field electron microscopy: Useful approximations', Acta
Cryst. A29 (1973), 529536.
69. J. M. Cowley, 'High
resolution dark-field electron microscopy. II. Short-range order in crystals', Acta
Cryst. A29 (1973), 537540.
70. P. L. Fejes, Sumio
Iijima and J. M. Cowley, 'Periodicity in thickness of electron microscopy
crystal lattice images', Acta Cryst. A29 (1973), 710714.
71. Shigeya Kuwabara and
J. M. Cowley, 'The effects of energy losses in aluminum on electron
diffraction intensities', J. Phys. Soc. Japan 34 (1973), 15751582.
72. Sumio Iijima, J. M.
Cowley and Gabrielle Donnay, 'High resolution electron microscopy of
tourmaline crystals', Tschermaks Mineralogische und Petrographishe Mitteilungen
20 (1973), 216224.
73. W. H. Massover and
J. M. Cowley, 'The ultrastructure of ferritin macromolecules. II. Lattice
structure of the core crystallites', Proc. Nat. Acad. Sci. 70 (1973),
38473851.
74. J. M. Cowley, W. H.
Massover and Bing K. Jap, 'The focussing of high resolution dark- field
electron microscope images', Optik 40 (1974), 4254.
75. J.
M. Cowley, David J. Smith and H. T. Pearce- Pearcy, 'The optimization of STEM
contrast for thick specimens', in 'Scanning Microscopy/1975', ed. Om Johari,
IIT Research Institute, Chicago (1975), 7178.
76. J. M. Cowley,
'Coherent and incoherent imaging in the scanning transmission electron
microscope', J. Phys. D: Appl. Phys. 8 (1975), L77L79.
77. J. M. Cowley, J. L.
Albain, G. G. Hembree, P. E. Hψjlund Nielsen, F.
A. Koch, J. D. Landry and H. Shuman, 'System for reflection electron
microscopy and electron diffraction at intermediate energies', Rev. Sci. Instr.
46 (1975), 826829.
78. David J. Smith and
J. M. Cowley, 'Aperture contrast in thick amorphous specimens using scanning
transmission electron microscopy', Ultramicroscopy 1 (1975), 127136.
79. J. M. Cowley and P.
E. Hψjlund Nielsen, 'Magnification variation in electron microscopy using diffracted
beams', Ultramicroscopy 1 (1975), 145150.
80. H. T. Pearce-Pearcy
and J. M. Cowley, 'On the use of energy filtering to increase the contrast of
STEM images of thick biological materials', Optik 44, 3 (1976),
273288.
81. P. E. Hψjlund
Nielsen and J. M. Cowley, 'Surface imaging using diffracted electrons', Surface
Sci. 54 (1976), 340354.
82. J. M. Cowley and
Bing K. Jap, 'The use of diffraction information to augment STEM imaging', in
'Scanning Electron Microscopy/1976', ed. Om Johari, IIT Research Institute, Chicago (1976), 377384.
83. J. M. Cowley,
'Diffraction by crystals with planar faults. I. General theory', Acta Cryst.
A32 (1976), 8387.
84. J. M. Cowley,
'Diffraction by crystals with planar faults. II. Magnesium fluorogermanate', Acta
Cryst. A32 (1976), 8891.
85. J. D. Landry, G. G.
Hembree, P. E. Hψjlund Nielsen and J. M. Cowley, 'SEM imaging of crystal
surfaces using diffracted beams', in 'Scanning Electron Microscopy/1976', ed.
Om Johari, IIT Research Institute, Chicago (1976), 239246.
86. A. J. Skarnulis,
Sumio Iijima and J. M. Cowley, 'Refinement of the defect structure of
'GeNb9O25', by high resolution electron microscopy', Acta
Cryst. A32 (1976), 799805.
87. J. M. Cowley, 'The
extension of scanning transmission electron microscopy by use of diffraction
information', Ultramicroscopy 1 (1976), 255262.
88. J. M. Cowley,
'Scanning transmission electron microscopy of thin specimens', Ultramicroscopy
2 (1976), 316.
89. Shigeya Kuwabara
and J. M. Cowley, 'Calculation of inelastic scattering effect in the bend
contour electron microscopic images of aluminum single crystals by n-slice
approximation', J. Phys. Soc. Japan 42 (1977), 19731979.
90. S. Iijima and J. M.
Cowley, 'Studies of ordering using HREM', J. de Phys. 38, Colloque C7
(1977), 135144.
91. P. M. Fields and J.
M. Cowley, 'Computed electron microscope images of atomic defects in F.C.C.
metals', Acta Cryst. A34 (1978), 103112.
92. Katsumichi Yagi and
J. M. Cowley, 'Electron microscopic study of ordering of potassium ions in
cubic KSbO3', Acta Cryst. A34 (1978), 625634.
93. J. C. H. Spence and
J. M. Cowley, 'Lattice imaging in STEM', Optik 50, 2 (1978), 129142.
94. J. M. Cowley and A.
Y. Au, 'Image signals and detector configurations in STEM', in 'Scanning
Electron Microscopy, 1978', ed. Om Johari, Scanning Electron Microscopy, Inc., Illinois, Vol. I (1978), 5360.
95. J. M. Cowley and
Yu-Jeng Chang, 'Diffraction by small crystals on a single crystal substrate',
Surface Sci. 72 (1978), 379389.
96. J. M. Cowley, 'Electron
Microscopy', Anal. Chem. 50 (1978), 76R80R.
97. J. M. Cowley and
Andrew Y. Au, 'Diffraction by crystals with planar faults. III. Structure
analysis using microtwins', Acta Cryst. A34 (1978), 738743.
98. J. M. Cowley, 'The
configuration of atom defects from High Resolution Transmission Electron
Microscopy', J. Nucl. Mat. 69 & 70 (1978), 228239.
99 G. G. Hembree and
J. M. Cowley, 'Electron channelling and microdiffraction from crystal
surfaces', in Scanning Electron Microscopy, 1979, Vol, I, ed. Om Johari, SEM
Inc., AMF O'Hare, Illinois (1979), 145152.
100. H. Brigette Krause,
J. M. Cowley and J. C. Wheatley, 'Short-range ordering in
PbMgNbO', Acta Cryst. A35 (1979), 10151017.
101. J. M. Cowley,
'Adjustment of STEM instrument by use of shadow images', Ultramicroscopy
4 (1979), 413418.
102. J. M. Cowley, J. C.
Wheatley and William L. Kehl, 'High resolution electron microscopy of LaPO4
catalysts', J. Catalysis (1979), 185194.
103. G. G. Hembree, J. M.
Cowley and M. A. Otooni, 'The oxidation of copper studied by electron
scattering techniques', Oxid. Met. 13 (1979), 331351.
104. J. M. Cowley and J.
C. H. Spence, 'Innovative imaging and microdiffraction in STEM', Ultramicroscopy
3 (1979), 433438.
105. J. M. Cowley and P.
M. Fields, 'Dynamical theory for electron scattering from crystal defects and
disorder', Acta Cryst. A35 (1979), 2837.
106. J. M. Cowley,
'Coherent interference in convergent beam electron diffraction and shadow
imaging', Ultramicroscopy 4 (1979), 435450.
107. J. M. Cowley and R.
E. Bridges, 'Phase and amplitude contrast in electron microscopy of stained
biological objects', Ultramicroscopy 4 (1979), 419429.
108. J. C. H. Spence, J.
M. Cowley and R. Gronsky, 'The effect of lens aberrations on lattice images of
spinodally decomposed alloys', Ultramicroscopy 4 (1979), 429433.
109. J. M. Cowley, 'High
resolution studies of crystals using STEM', Chem. Scripta 14
(19781979), 3338.
110. J. M. Cowley,
'Direct imaging of atoms in crystals and molecules: Status and prospects for physics',
Chem. Scripta 14 (197879), 279285.
111. G. Schiffmaker, H.
Dexpert, P. Caro and J. M. Cowley, 'Elliptical electron diffraction
patterns from thin films of 'turbostratic' graphite', J. Microsc. Spect.
Elec. 5 (1980), 729734.
112. J. M. Cowley, 'A
facility for high resolution electron microscopy', B. Electron Microsc. Soc.
Am. 10, 1 (1980), 2024.
113. J. M. Cowley,
'Interference effects in a STEM instrument', Micron 11 (1980), 229233.
114. J. M. Cowley, M.
Strahm and J. H. Butler, 'Recording and processing of STEM images', Micron
11 (1980), 285286.
115. J. M. Cowley, 'The
prospects for high resolution imaging', Micron 11 (1980), 223227.
116. J. M. Cowley,
'Optical processing of diffraction information in STEM', in Scanning Electron
Microscopy/1980, ed. Om Johari, SEM Inc., AMF O'Hare, Illinois, Vol. 1 (1980),
6172.
117. J. M. Cowley and M.
Disko, 'Fresnel diffraction in a coherent convergent electron beam', Ultramicroscopy
5 (1980), 469477.
118. Fumio Watari and J.
M. Cowley, 'The study of oxide formation on (001) (011) (111) and (113)
surfaces of Cr thin films using STEM- microdiffraction methods', Surface
Sci. 105 (1981), 240264.
119. J. M. Cowley and D.
J. Walker, 'Reconstruction from in-line holograms by digital processing', Ultramicroscopy
6 (1981), 7176.
120. P. S. Turner and J.
M. Cowley, 'STEM and CTEM observations of interference between Laue- and
Bragg-diffracted electrons in images of polyhedral crystals', Ultramicroscopy
6 (1981), 125138.
121. R. A. Roy, R.
Messier and J. M. Cowley, 'Fine structure of gold particles in thin films prepared
by metal insulator co-sputtering', Thin Solid Films 79 (1981), 207215.
122. J. M. Cowley,
'Coherent interference effects in STEM and CBED', Ultramicroscopy 7
(1981), 1926.
123. J. M. Cowley and J.
C. H. Spence, 'Convergent beam electron microdiffraction from small crystals',
Ultramicroscopy 6 (1981), 359366.
124. J. M. Cowley,
'Coherent convergent beam microdiffraction', Kristallografiya 26 (1981)
965973 (in Russian); Soviet Phys.Crystallog. 26 (1981), 549533 (in
English).
125. J. M. Cowley,
'Electron Microdiffraction studies of the potential field at crystal surfaces',
Ultramicroscopy 7 (1981), 181188.
126. P. Goodman, J. M.
Cowley and A. Higgs, 'Inelastic scattering contrast in beam-rocking electron
diffraction experiments', Ultramicroscopy 6 (1981), 377382.
127. J. M. Cowley and R.
A. Roy, 'Microdiffraction of gold microcrystals', in Scanning Electron
Microscopy 1981, ed. Om Johari, SEM, Inc., AMF O'Hare (Chicago) (1982), 143152.
128. J. M. Cowley,
'Surface energies and surface structure of small crystals studied by use of a
STEM instrument', Surface Sci. 114 (1982), 587600.
129. J. M. Cowley,
'Energy losses of fast electrons at crystal surfaces', Phys Rev. B 25, 2
(1982), 14011404.
130. J. M. Cowley, 'The
accomplishments and prospects of high resolution imaging methods,' Ultramicroscopy
8 (1982), 112.
131. Jing Zhu and J. M.
Cowley, 'Microdiffraction from anti-phase boundaries in Cu3Au', Acta Cryst.
A38 (1982), 718724.
132. J. M. Cowley,
'Microdiffraction, STEM imaging and ELS at crystal surfaces', Ultramicroscopy
9 (1982), 231236.
133. P. R. Buseck and J.
M. Cowley, 'Modulated and intergrowth structures in minerals and electron
microscopy methods for their study', Am. Mineral. 68 (1983), 1840.
134. J. M. Cowley,
'Scanning transmission electron diffraction and microdiffraction techniques',
B. Mater. Sci. 6 (1984), 477490.
135. Jing Zhu and J. M.
Cowley, 'Microdiffraction from stacking faults and twin boundaries in F.C.C.
crystals', J. Appl. Cryst. 16 (1983), 171175.
136. J. M. Cowley, 'The
STEM approach to the imaging of surfaces and small particles', J. Microsc.
129 (1983), 253261.
137. J. M. Cowley,
'Microdiffraction in a STEM instrument and application to surface structures',
in Scanning Electron Microscopy/1982, ed. Om Johari, SEM Inc., Chicago, Vol. 1
(1983), 5160.
138. J. M. Cowley and
Z.-C. Kang, 'STEM imaging and analysis of surfaces', Ultramicroscopy
11 (1983), 131140.
139. Tung Hsu and J. M.
Cowley, 'Reflection electron microscopy (REM) of F.C.C. metals', Ultramicroscopy
11 (1983), 239250.
140. J. H. Butler and J.
M. Cowley, 'Phase contrast imaging using a scanning transmission electron
microscope', Ultramicroscopy 12 (1983), 3950.
141. W. Bryan Monosmith
and J. M. Cowley, 'Pattern recognition techniques for the analysis of electron
microdiffraction patterns', Ultramicroscopy 12 (1983), 5158.
142. J. M. Cowley, 'STEM
imaging of thick specimens with off-axis detectors', J. Electron Micr.
Tech. 1 (1984), 8394.
143 W. Bryan Monosmith
and J. M. Cowley, 'Electron microdiffraction from very small gold particles', Ultramicroscopy
12 (1984), 177184.
144. C.-S. Tan and J. M.
Cowley, 'Surface potential study of Au(111) surfaces', Ultramicroscopy
12 (1984), 333344.
145. J. M. Cowley and K.
D. Neumann, 'The alignment of gold particles on MgO crystal surfaces', Surface
Sci. 145 (1984), 301312.
146. J. M. Cowley,
'Microdiffraction and STEM of interfaces', Ultramicroscopy 14 (1984),
2736.
147. Elizabeth A. Lodge
and J. M. Cowley, 'The surface diffusion of silver under high resolution
imaging conditions', Ultramicroscopy 13 (1984), 215226.
148. Tung Hsu, Sumio
Iijima and J. M. Cowley, 'Atomic and other structures of cleaved GaAs (111)
surfaces', Surface Sci. 137 (1984), 551569.
149. J. M. Cowley,
'Nanodiffraction: electron diffraction from nanometer size regions', Denshi-Kembikyo
18 (1984), 128133 (in Japanese).
150. J. M. Cowley,
Mohamed A. Osman and P. Humble, 'Nanodiffraction from platelet
defects in diamond', Ultramicroscopy 15 (1984), 311318.
151. J. M. Cowley and
Lian-mao Peng, 'The image contrast of surface steps in reflection electron
microscopy', Ultramicroscopy 16 (1985), 5967.
152. C. Elibol, H.-J. Ou,
G. G. Hembree and J. M. Cowley, 'An improved instrument for medium
energy electron diffraction and microscopy of surfaces', Rev. Sci. Instr.
56 (1985), 12151219.
153. J. M. Cowley, 'High
resolution electron microscopy and microdiffraction', Ultramicroscopy
18 (1985), 1117.
154. Jing Zhu, H. Q. Ye
and J. M. Cowley, 'Effect of anti-phase domain boundaries on microdiffraction:
Computer simulation', Ultramicroscopy 18 (1985), 111116.
155. N. Tanaka and J. M.
Cowley, 'Studies of planar defects in silver plate-like crystals by CBED and
HRTEM techniques', Mater. Res. 41 (1985), 155162.
156. Tung Hsu and J. M.
Cowley, 'Surface characterization by reflection electron microscopy (REM)', Mater.
Res. 41 (1985), 121127.
157. Guo-You Fan and J.
M. Cowley, 'Auto-correlations analysis of high resolution electron micrographs
of near-amorphous thin films', Ultramicroscopy 17 (1985), 345355.
158. N. Tanaka and J. M.
Cowley, 'High resolution electron microscopy of disordered lithium ferrites', Ultramicroscopy
17 (1985), 365377.
159. Jing Zhu and J. M.
Cowley, 'Study of early- stage precipitation in Al-4%Cu by microdiffraction
and STEM', Ultramicroscopy 18 (1985), 419426.
160. P. A. Bennett, H.-J.
Ou, C. Elibol and J. M. Cowley, 'Domain structure of the
Si(111) 2x1 surface studied by reflection electron microscopy', J. Vac. Sci.
Technol. A3 (1985), 16341635.
161. J. M. Cowley, 'The
future of high resolution electron microscopy', Ultramicroscopy 18
(1985), 463468.
162. J. M. Cowley and Z.
L. Wang, 'Defocussed dark field images of crystal surfaces', Ultramicroscopy
19 (1986), 217223.
163. J. M. Cowley,
'Electron diffraction phenomena observed with a high resolution STEM
instrument', J. Electron Micr. Tech. 3 (1986), 2544.
164. T. Tanji and J. M.
Cowley, 'Interactions of electron beams with surface of MgO crystals', Ultramicroscopy
17 (1985), 287302.
165. J. A. Lin and J. M.
Cowley, 'Calibration of the operating parameters for an HB5 STEM Instrument', Ultramicroscopy
19 (1986), 3142.
166. J. A. Lin and J. M.
Cowley, 'Reconstruction from in-line electron holograms by digital processing',
Ultramicroscopy 19 (1986), 179190.
167. L. M. Peng and J. M.
Cowley, 'Dynamical diffraction calculations for RHEED and REM', Acta Cryst.
A42 (1986), 545552.
168. N. Tanaka, J. M.
Cowley and K. Ohshima, 'High resolution electron microscopy observations of
disordered Au15at% Mn alloys', Acta Cryst. A43 (1987), 4148.
169. S.-Y. Zhang and J.
M. Cowley, 'HREM and nanodiffraction study of MgO-Al Interface', Thin Solid
Films 148 (1987), 301310.
170. Z. L. Wang and J. M.
Cowley, 'Surface plasmon excitation for supported metal particles', Ultramicroscopy
21 (1987), 7794.
171. G. Y. Fan and J. M.
Cowley, 'The simulation of high-resolution images of amorphous thin films', Ultramicroscopy
21 (1987), 125130.
172. J. A. Venables, D.
J. Smith and J. M. Cowley, 'HREM, STEM, REM, STEM - and STM', Surface Sci.
181 (1986), 235249.
173. J. A. Lin and J. M.
Cowley, 'Aberration analysis by three-beam interferograms', Appl. Optics
25 (1986), 22452246.
174. J. M. Cowley,
'Electron microscopy and surface structure', Progr. Surface Sci. 21
(1986), 209250.
175. Tung Hsu, J. M.
Cowley, L.-M. Peng and H.‑J. Ou, 'Reflection electron microscopy
methods for the study of surface structure', J. Microsc. 146
(1987), 1727.
176. G.-Y. Fan, J. M.
Cowley and J. C. H. Spence, Comment on 'Submicrocrystallites and orientational
proximity effects', Phys. Rev. Lett. 58 (1987), 282283.
177. C. Mory, C. Colliex
and J. M. Cowley, 'About an optimum defocus for STEM imaging and
microanalysis', Ultramicroscopy 21 (1987), 171177.
178. N. Tanaka and J. M.
Cowley, 'Electron microscope imaging of short range order in disordered
alloys', Acta Cryst. A43 (1987), 337346.
179. L. M. Peng and J. M.
Cowley, 'A geometric analysis of surface resonance conditions in RHEED', J.
Electron Micr. Tech. 6 (1987), 4353.
180. J. M. Cowley and D.
J. Smith, 'The present and future of high resolution electron microscopy', Acta
Cryst. A43 (1987), 593612.
181. J. M. Cowley, 'High
resolution imaging and diffraction studies of crystal surfaces', J. Electron
Microsc. 36 (1987), 7281.
182. H.-J. Ou and J. M.
Cowley, 'SREM of MgO crystal surface structure and in-situ deposited metallic
particles on MgO surface', Ultramicroscopy 22 (1987), 207216.
183. Z.-L. Wang and J. M.
Cowley, 'Generation of surface plasmon excitation of supported metal particles
by an external electron beam', Ultramicroscopy 21 (1987), 347366.
184. Z.-L. Wang and J. M.
Cowley, 'Excitation of the supported metal particles surface plasmon with
external electron beam', Ultramicroscopy 21 (1987). 335346.
185. M. Pan, J. M. Cowley
and I. Y. Chan, 'The structure of Pt particles on a-Al2O3', J. Appl. Cryst. 20
(1987), 300305.
186. Z.-L. Wang and J. M.
Cowley, 'Size and shape dependence of the surface plasmon frequencies for
supported metal particle systems', Ultramicroscopy 23 (1987), 97108.
187. Z. L. Wang, P. Lu
and J. M. Cowley, 'Electron resonance channeling on crystal surfaces in
reflection high energy electron diffraction geometry', Ultramicroscopy
23 (1987), 205222.
188. J. M. Cowley,
'Imaging and diffraction on the atomic scale', Aust. Physicist 24
(1987), 264268.
189. L.-M. Peng and J. M.
Cowley, 'Diffraction contrast in reflection electron microscopy. I. Screw
dislocation', Micron Microsc. Acta 18 (1987), 171178.
190. L.-M. Peng, J. M.
Cowley and Tung Hsu, 'Diffraction contrast in reflection electron microscopy.
II. Surface steps and dislocations under the surface', Micron Microsc. Acta
18 (1987), 179186.
191. J. M. Cowley, 'High
resolution electron microscopy', Ann. Rev. Phys. Chem. 38 (1987), 5788.
192. M. Pan, J. M. Cowley
and R. Garcia, 'STEM and microdiffraction studies of Rh/CeO2', Micron
Microsc. Acta 18 (1987), 165169.
193. J. Liu and J. M.
Cowley, 'High resolution SEM of surface reactions', Ultramicroscopy 23
(1987), 463472.
194. Jing Zhu, L.-M. Peng
and J. M. Cowley, 'Effects of the coherence of illumination in electron microdiffraction
pattern intensities', J. Electron Micr. Tech. 7 (1987), 177183.
195. J. M. Cowley and R.
J. Plano, 'A microdiffraction study of gold-ruthenium catalyst particles', J.
Catalysis 108 (1987), 199207.
196. H.-J. Ou and J. M.
Cowley, 'Study of freshly deposited metallic particles on MgO crystal surfaces
by scanning reflection electron microscopy', Ultramicroscopy 23 (1987),
263270.
197. Z.-L. Wang and J. M.
Cowley, 'Reflection electron energy-loss spectroscopy (REELS): a technique for
the study of surfaces', Surface Sci. 193 (1988), 501512.
198. J. Liu and J. M.
Cowley, 'High resolution SEM in a STEM instrument', Scanning Microscopy
2 (1988), 6581.
199. L.-M. Peng and J. M.
Cowley, 'Errors arising from numerical use of the Mott formula in electron
image simulation', Acta Cryst. A44 (1988), 15.
200. G. Y. Fan and J. M.
Cowley, 'Assessing the information content of HREM images', Ultramicroscopy
24 (1988), 4960.
201. Z. L. Wang and J. M.
Cowley, 'Atomic inner shell excitations for EELS in the reflection mode', J.
Micros Spectros. Electr. 13 (1988), 184204.
202. L. M. Peng and J. M.
Cowley, 'A multislice approach to the RHEED and REM calculation', Surface
Sci. 199 (1988), 609622.
203. L. M. Peng and J. M.
Cowley, 'Experimental studies of surface resonance scattering processes in
RHEED', Surface Sci. 201 (1988), 559571.
204. M. Pan and J. M.
Cowley, 'Computer-simulated electron microdiffraction patterns from MgO
crystal surfaces', Ultramicroscopy 26 (1988), 205216.
205. Z. L. Wang and J. M.
Cowley, 'REELS and RHEED characterizations of electron resonance channelling
in crystal surfaces', Ultramicroscopy 26 (1988), 233238.
206. L. M. Peng, J. M.
Cowley and N. Yao, 'The observation of surface resonance effects in RHEED
patterns', Ultramicroscopy 26 (1988), 189194.
207. L. M. Peng and J. M.
Cowley, 'Surface resonance effects and beam convergence in REM', Ultramicroscopy
26 (1988), 161167.
208. L. M. Peng and J. M.
Cowley, 'Diffuse diffraction spots in RHEED patterns', Ultramicroscopy
26 (1988), 227232.
209. L.-M. Peng and J. M.
Cowley, 'EELS analysis of surface-channelled electrons', Surface Sci.
204 (1988), 555567.
210. H. J. Ou and J. M.
Cowley, 'The surface reaction of Pd/MgO studied by scanning reflection
electron microscopy', Phys. Status Solidi 107 (1988), 719729.
211. J. M. Cowley, 'High
resolution electron microscopy of the solid-vacuum interface', J. Vac. Sci.
Technol. A6, 3 (1988), 1.
212. J. M. Cowley,
'Electron microscopy of crystals with time-dependent perturbations', Acta Cryst.
A44 (1988), 847853.
213. J.
Liu and J. M. Cowley, 'Contrast and resolution of secondary electron images in
a scanning transmission electron microscope', Scanning Microscopy 2, 4
(1988), 19571970.
214. Z. L. Wang, J. Liu,
Ping Lu and J. M. Cowley, 'Electron resonance reflections from perfect crystal
surfaces and surfaces with steps', Ultramicroscopy 27 (1988), 101112.
215. H.-J. Ou, S.-C.Y.
Tsen, K. T. Tsen, J. M. Cowley, J. I. Chyi, A. Salvador
and H. Morkoc, 'Determination of the local Al concentration in Alx
Ga1-xAs-GaAs quantum well structures using the (200) diffraction intensity
obtained with a 10Δ electron beam', Appl. Phys. Lett. 54, 15 (1989),
14541456.
216. Nan Yao, Z. L. Wang
and J. M. Cowley, 'REM and REELS identifications of atomic terminations at
a-Alumina (011) surface', Surface Sci. 208 (1989), 533549.
217. Takayoshi Tanji,
Hideki Masaoka, Jhota Ito, Keiji Yada and J. M. Cowley, 'Charging effect on the
HRTEM imaging of small MgO crystals', Ultramicroscopy 27 (1989),
223232.
218. J. M. Cowley and
H.-J. Ou, 'Observation of microdiffraction patterns with a dedicated STEM
instrument', J. Electron Micr. Tech. 11 (1989), 143154.
219. J. M. Cowley,
'Observation of surface channelling phenomena with a STEM instrument', Ultramicroscopy
27 (1989), 319329.
220. J. Konnert, P.
D'Antonio, J. M. Cowley, A. Higgs and H.-J. Ou, 'Determination of
atomic positions using electron nanodiffraction patterns from overlapping
regions: Si[110]', Ultramicroscopy 30 (1989), 371384.
221. Z. L. Wang, J. Liu
and J. M. Cowley, 'Electron inelastic plasmon scattering and its resonance
propagation at crystal surfaces in RHEED', Acta Cryst. A45 (1989),
325332.
222. L.-M. Peng, J. M.
Cowley and T. Hsu, 'Reflection electron imaging of free surfaces and
surface/dislocation interactions', Ultramicroscopy 29 (1989), 135146.
223. L.-M. Peng and J. M.
Cowley, 'Thermal diffuse scattering and REM image-contrast preservation', Ultramicroscopy
29 (1989), 168174.
224. J. M. Cowley,
'Imaging and analysis of surfaces with high spatial resolution', J. Vac.
Sci. Technol. A7 (1989), 8994.
225. M. Pan, J. M. Cowley
and J. C. Barry, 'Coherent electron microdiffraction from small metal
particles', Ultramicroscopy 30 (1989), 385394.
226. Nan Yao and J. M.
Cowley, 'The parabolas and circles in RHEED patterns', Ultramicroscopy
31 (1989), 149157.
227. G. G. Hembree, P. A.
Crozier, J. S. Drucker, M. Krishnamurthy, J. A. Venables and
J. M. Cowley, 'Biassed secondary electron imaging in a UHV-STEM', Ultramicroscopy
31 (1989), 111115.
228. Z. L. Wang, J. Liu
and J. M. Cowley, 'Sensitivity of the ELNES in REELS to the beam reductions at
the TiO2 (110) surfaces', Surface Sci. 216 (1989), 528538.
229. Z. L. Wang and J. M.
Cowley, 'Simulating high-angle annular dark-field STEM images including
inelastic thermal diffuse scattering', Ultramicroscopy 31 (1989),
437454.
230. J. M. Cowley,
'Surface channelling effects in electron holograms', Ultramicroscopy 31
(1989), 223232.
231. Z. L. Wang and J. M.
Cowley, 'Dynamic theory of high-angle annular dark field STEM lattice images
for a Ge/Si interface', Ultramicroscopy 32 (1990), 275289.
232. J. Liu and J. M.
Cowley, 'High Angle ADF and High resolution SE imaging of supported catalyst
clusters', Ultramicroscopy 34 (1990), 119128.
233. M. Pan, J. M. Cowley
and I. Y. Chan, 'HREM imaging of small Pt clusters dispersed in Y‑zeolites',
Catalyst Lett. 5 (1990), 112.
234. M. Pan, J. M. Cowley
and I. Y. Chan, 'Study of high dispersed Pt in Y-zeolites by STEM and electron
micro-diffraction', Ultramicroscopy 34 (1990), 93101.
235. H.-J. Ou, J. M.
Cowley, J. I. Chyi, A. Salvador and H. Morkoc, 'Microanalysis on the (200)
diffraction intensity to determine the Al concentrations for AlGaAs-GaAs MQWS
structures', J. Appl. Phys. 67, 2 (1990), 698704.
236. N. Yao and J. M.
Cowley, 'Electron diffraction conditions and surface imaging in reflection
electron microscopy', Ultramicroscopy 33 (1990), 237254.
237. J. M. Cowley, 'High
Resolution side-band holography with a STEM Instrument', Ultramicroscopy
34 (1990), 293297.
238. M.
Gajdardziska-Josifovska and J. M. Cowley, 'Brillouin zones and Kikuchi lines by
crystals under electron channelling conditions', Acta Cryst. A47 (1991),
7482.
239. J. Liu and J. M.
Cowley, 'Imaging with high- angle scattered electrons and secondary electrons
in the STEM', Ultramicroscopy 37 (1991), 5071.
240. M. Gajdardziska-Josifovska,
P. A. Crozier and J. M. Cowley, 'A (3x3) R30° reconstruction on annealed (111)
surfaces of MgO', Surface Sci. Lett. 248 (1991), L259L264.
241. P. Lu, J. Liu and J.
M. Cowley, 'Theoretical and experimental studies of electron resonance effects
in reflection high energy electron diffraction', Acta Cryst. A47
(1991), 317327.
242. Nan Yao and J. M.
Cowley, 'Observation of double-line contrast in surface imaging', Micros.
Res. Tech. 20 (1992), 413425.
243. Godfrey C. Ndubuisi,
J. Liu and J. M. Cowley, 'Characterization of the annealed (0001)
surface of sapphire (_‑Al2O3) and interaction with silver by REM and
SREM', Micros. Res. Tech. 20 (1992), 439449.
244. P. A. Crozier, M.
Gajdardziska-Josifovska and J. M. Cowley, 'Preparation and characterization of
MgO surfaces by reflection electron microscopy', Micros. Res. Tech. 20
(1992), 426438.
245. J. Liu, Y. Cheng, J.
M. Cowley and M. B. Stearns, 'High-angle annular dark-field microscopy of Mo/Si
multilayer structures', Ultramicroscopy 40 (1992), 352364.
246. Godfrey C. Ndubuisi,
J. Liu and J. M. Cowley, 'Stepped surfaces of sapphire (a-Al2O3) with low
Miller indices', Micros. Res. Tech. 21 (1992), 1022.
247. J. M. Cowley and Yi
Huang, 'De-channelling contrast in annular dark-field STEM', Ultramicroscopy
40 (1992), 171180.
248. J. M. Cowley,
'Resolution limitation in the electron microscopy of surfaces', Ultramicroscopy
47 (1992), 187198.
249. J. Liu, L. Wang and
J. M. Cowley, 'Alumina- induced reconstruction on annealed (001) surfaces of
rutile', Surface Sci. 268 (1992), L293L299.
250. J. M. Cowley,
'Twenty forms of electron holography', Ultramicroscopy 41 (1992),
335348.
251. Feng Tsai and J. M.
Cowley, 'Observation of ferroelectric domain boundaries in BaTiO3 single
crystals by reflection electron microscopy (REM)', Ultramicroscopy 45
(1992), 4353.
252. Feng Tsai, Victoria Khiznichencko and J. M. Cowley, 'High resolution electron microscopy of
90° ferroelectric domain boundaries in BaTiO3 and
Pb (Zr0.52 Ti0.48)O3', Ultramicroscopy 45 (1992), 5563.
253. M. A. Gribelyuk and
J. M. Cowley, 'Computer analysis of side-band holography in STEM', Ultramicroscopy
45 (1992), 103113.
254. M. A. Gribelyuk and
J. M. Cowley, 'Determination of the imaging conditions in off-axis side-band
STEM holography', Ultramicroscopy 45 (1992), 115125.
255. Yi Huang and J. M.
Cowley, 'A study of Cu3Au (110) surface structure by RHEED', Surface
Sci. 285 (1993), 4258.
256. M. Gajdardziska, P.
A. Crozier, M. R. McCartney and J. M. Cowley, 'Ca segregation and
step modification on cleaved and annealed MgO (100) surfaces', Surface Sci.
284 (1993), 186199.
257. J. Liu and J. M.
Cowley, 'Scanning reflection electron microscopy and associated techniques for
surface studies', Ultramicroscopy 48 (1993), 381416.
258. Mingqi Liu and J. M.
Cowley, 'Particle/dislocation interactions in dispersion strengthened tungsten
alloy at ultra-high temperatures', Scripta Metall. Mater. 28 (1993),
307312.
259. Mingqi Liu and J. M.
Cowley, 'Hafnium carbide growth behavior and its relationship to the
dispersion hardening in tungsten at high temperatures', Mater. Sci. Eng. A160 (1993), 159167.
260. J. M.
Cowley,'Configured detectors for STEM imaging of thin specimens', Ultramicroscopy
49 (1993), 413.
261. M. A. Gribelyuk and
J. M. Cowley, 'Determination of experimental imaging conditions for off-axis
transmission electron holography', Ultramicroscopy 50 (1993), 2940.
262. J. C. H. Spence, J.
M. Cowley and J. M. Zuo, 'Comment on: Electron holographic study of ferroelectric
domain walls', Appl. Phys. Lett. 62 (1993), 24462447.
263. F. Tsai and J. M.
Cowley, 'Observation of ferroelectric domain boundaries in BaTiO3 by
transmission and reflection electron microscopy', Ferroelectrics 140
(1993), 203210.
264. S. Kraut and J. M.
Cowley, 'A simplified mode of differential phase contrast Lorentz microscopy', Microsc.
Res. Tech. 25 (1993), 341345.
265. Y. Huang and J. M.
Cowley, 'Structure of sulfur-adsorbed Cu3Au(110) surface', Surface
Sc. 289 (1993), 340356.
266. J. M. Cowley and J.
Liu, 'Contrast and resolution in REM, SEM and SAM', Surface Sci. 298
(1993), 456467.
267. J. M. Cowley,
'Electron holography and holographic diffraction in surface science', Surface
Sci. 298 (1993), 336344.
268. J. Liu and J. M.
Cowley, 'High resolution scanning transmission electron microscopy', Ultramicroscopy
52 (1993), 335346.
269. Feng Tsai and J. M.
Cowley, 'Observation of planar defects by reflection electron microscopy', Ultramicroscopy
52 (1993), 400403.
270. Marian Mankos, J. M.
Cowley, R. V. Chamberlin, M. R. Scheinfein and M. B.
Stearns, 'Scanning transmission electron microscopy of thin magnetic films', IEEE
Trans. Magnetics 30 (1993), 720722.
271. L. Wang, J. Liu and
J. M. Cowley, 'Studies of single crystal TiO2(001) and (100)
surfaces by reflection high energy electron diffraction and reflection electron
microscopy', Surface Sci. 302 (1994), 141157.
272. Yimei Zhu and J. M.
Cowley, 'Three-dimensional structural modulation in doped YBa2Cu3O7-d', Phil. Mag. A 69 (1994),
397408.
273. J. M. Cowley and M.
A. Gribelyuk, 'High resolution coherent imaging and holography in STEM', Microsc.
Soc. Am. B. 24 (1994), 438450.
274. Ming-qi Liu and J.
M. Cowley, 'Structure of carbon nanotubes studied by HRTEM and
nanodiffraction', Ultramicroscopy 53 (1994), 333342.
275. Ming-qi Liu and J.
M. Cowley, 'Growth behavior and growth defects of carbon nanotubes', Mater.
Sci. Eng. A185 (1994), 131140.
276. J. M. Cowley and
Ming-qi Liu, 'The structure of carbon nanotubes impregnated with yttrium', Micron
25 (1994), 5361.
277. Ming-qi Liu and J.
M. Cowley, 'Structures of the helical carbon nanotubes', Carbon 32
(1994), 393403.
278. L. Wang and J. M.
Cowley, 'Electron channelling effects at high incident angles in convergent
beam reflection high energy electron diffraction', Ultramicroscopy 55
(1994), 228240.
279. Tung Hsu and J. M.
Cowley, 'Study of twinning with the reflection electron microscopy (REM)', Ultramicroscopy
55 (1994), 302307.
280. Marian Mankos, M. R.
Scheinfein and J. M. Cowley, 'Absolute magnetometry at nm transverse
spatial resolution: STEM holography of thin cobalt films', J. Appl. Phys.
75 (1994), 74187422.
281. J. M. Cowley, M. Q.
Liu, B. L. Ramakrishna, T. S. Peace, A. K. Wertsching and M. R. Pena, 'A new type of
metal-fulleride structure: C60Pd3', Carbon 32
(1994), 746748.
282. Feng Tsai and J. M.
Cowley, 'Thickness dependence of ferroelectric domains in thin crystalline
films', Appl. Phys. Lett. 65 (1994), 19061908.
283. J. M. Cowley, M.
Mankos, M. R. Scheinfein and Z. J. Yang, 'Absolute magnetometry of thin cobalt
films and Co/Cu multilayer structures with nanometer spatial resolution', IEEE
Trans. Magnetics 30, 6 (1994), 44974499.
284. M.
Gajdardziska-Josifovska, J. K. Weiss and J. M. Cowley, 'Studies of Mo/Si
multilayers with coherent electron beams', Ultramicroscopy 58 (1995),
6578.
285. Marian Mankos, A. A.
Higgs, M. R. Scheinfein and J. M. Cowley, 'Far-out-of-focus electron
holography in a dedicated FEG STEM', Ultramicroscopy 58 (1995), 8796.
286. J. M. Cowley, M. S.
Hansen and S. Y. Wang, 'Imaging modes with an annular detector in STEM', Ultramicroscopy
58 (1995), 1824.
287. Shi-Yao Wang and J.
M. Cowley, 'Shadow images for in-line holography in a STEM instrument', Micros.
Res. Tech. 30 (1995), 181192.
288. Yi Huang, M.
Gajdardziska-Josifovska and J. M. Cowley, 'REM in a UHV TEM for the
observation of dynamic phase transformation processes on the Cu3Au(111)
surface', Ultramicroscopy 57 (1995), 391408.
289. Mingqi Liu and J. M.
Cowley, 'Encapsulation of lanthanum carbide in carbon nanotubes and carbon
nanoparticles', Carbon 33 (1995), 225232.
290. J. M. Cowley,
'Chromatic coherence and inelastic scattering in electron holography', Ultramicroscopy
57 (1995), 327331.
291. Mingqi Liu and J. M.
Cowley, 'Encapsulation of manganese carbides within carbon nanotubes and
nanoparticles', Carbon 33 (1995), 749756.
292. Yi Huang and J. M.
Cowley, 'SEM and SAM study of sulfur segregation on a Cu3Au(110) surface', Surface
Sci. 328 (1995), 277286.
293. Marian Mankos, J. M.
Cowley and M. R. Scheinfein, 'Absolute magnetometry using electron
holography: Magnetic superlattices and small particles', MRS Bulletin
20, 10 (1995), 4548.
294. M. Mankos, M. R.
Scheinfein and J. M. Cowley, 'Absolute magnetometry of
small particles using electron holography', IEEE Trans. Magnetics 31
(1995), 37963798.
295. R.-J. Liu and J. M.
Cowley. 'Dark-Field and Marginal Imaging with a Thin-Annular Detector in STEM',
J. Micros. Soc. Am. 2 (1996), 919.
296. J. M. Cowley and
Scott D. Packard, 'Coherent nanodiffraction from phase objects: Carbon
nanotubes', Ultramicroscopy 63 (1996), 3947.
297. J. M. Cowley, M.
Mankos and M. R. Scheinfein, 'Greatly-defocused, point- projection,
off-axis electron holography', Ultramicroscopy 63 (1996),
133147.
298. Marian Mankos, J. M.
Cowley and M. R. Scheinfein, 'Quantitative micromagnetics at high
spatial resolution using electron holography', Phys. Status Solidi A 154
(1996), 469504.
299. J. M. Cowley, V. I.
Merkulov and J. S. Lannin, 'Imaging of light-atom nanocrystals with a thin
annular detector in STEM', Ultramicroscopy 65 (1996), 6170.
300. Yi Huang and John M.
Cowley, 'Contact potential contrast in SEM images observed on sulfur-adsorbed
Cu3Au (110) surfaces', Ultramicroscopy
66 (1996), 211220.
301. J. M. Cowley, M.
Mankos and M. R. Scheinfein, 'Quantitative
micromagnetics: electron holography of magnetic thin films and multilayers', IEEE
Trans. Magnetics 32, 5 (1996), 41504155.
302. J. M. Cowley, Pavel
Nikolaev, Andreas Thess and Richard E. Smalley, 'Electron nanodiffraction
study of carbon single-walled nanotube ropes', Chem. Phys. Lett. 265
(1997), 379384.
303. A. Amali, P. Rez and
J. M. Cowley, 'High- angle annular dark-field imaging of stacking faults', Micron
28 (1997), 8994.
304. J. M. Cowley and F.
A. Sundell, 'Nanodiffraction and dark-field STEM characterization of
single-walled carbon nanotube ropes', Ultramicroscopy 68 (1997), 112.
305. J. M. Cowley, J. C.
H. Spence and Valery V. Smirnov, 'The enhancement of electron microscope
resolution by use of atomic focusers', Ultramicroscopy 68 (1997),
135148.
306. J. M. Cowley,
'Applications of STEM instruments for surface studies', Surface Rev. Lett.
4, 3 (1997), 567575.
307. Michael Sanchez and
J. M. Cowley, 'The imaging properties of atomic focusers', Ultramicroscopy
72 (1998), 213222.
308. J. M. Cowley, R. E.
Dunin-Borkowski and Michele Hayward, 'The contrast of images formed by atomic
focusers', Ultramicroscopy 72 (1998), 223232.
309. Max V. Siderov,
Michael D. McKelvy, John M. Cowley and William S. Glaunsinger, 'Novel
guest-layer behavior of mercury titanium disulfide
intercalates', Chem. Mater. 10 (1998), 32903293.
310. R. E.
Dunin-Borkowski and J. M. Cowley, 'Simulations for imaging with atomic focusers',
Acta Cryst. A55 (1999), 119126.
311. J. M. Cowley, Newton
Ooi and R. E. Dunin- Borkowski, 'Moirι patterns in electron microscopy with
atomic focuser crystals', Acta Cryst. A55 (1999), 533542.
312. Dawn E. Janney, J.
M. Cowley and Peter R. Buseck, 'Transmission electron microscopy of synthetic
2-and 6-line ferrihydrite', Clays Clay Miner. 48 (2000), 111119.
313. J. M. Cowley,
'Atomic-focuser imaging in electron nanodiffraction from carbon nanoshells', Ultramicroscopy
81 (2000), 4755.
314. Dawn E. Janney, J.
M. Cowley and Peter R. Buseck, 'Structure of synthetic 2-line ferrihydrite by
electron nanodiffraction', Am. Mineral. 85 (2000), 11801187.
315. J. M. Cowley and J.
B. Hudis, 'Atomic- focuser imaging by graphite crystals in carbon nanoshells',
Microsc. Microanal. 6 (2000), 429436.
316. J. M. Cowley,
'Electron holography with atomic focusers', Phys. Rev. Lett. 84, 16
(2000), 36183621.
317. J. M. Cowley and
Ching-Hwa Kiang, 'The structures of near-spherical carbon nano- shells', Carbon
38 (2000), 14371444.
318. J. M. Cowley, Dawn
E. Janney, R. C. Gerkin and Peter R. Buseck, 'The structure of ferritin cores
determined by electron nanodiffraction', J. Struct. Biol. 131 (2000),
210216.
319. V. V. Kovalevski,
Peter R. Buseck and J. M. Cowley, 'Comparison of carbon in shungite rocks to
other natural carbons: an X-ray and TEM study', Carbon 39 (2001),
243256.
320. J. M. Cowley,
'Comments on ultra-high resolution STEM', Ultramicroscopy 87 (2001),
14.
321. Dawn E. Janney, J.
M. Cowley and Peter R. Buseck, 'Structure of synthetic 6-line ferrihydrite by
electron nanodiffraction', Am. Mineral. 86 (2001), 327335.
322. J. M. Cowley and
Jamie Winterton, 'Ultra- high-resolution electron microscopy of carbon
nanotube walls', Phys. Rev. Lett. 87, 1 (2001), 14.
323. J. M. Cowley, 'STEM
imaging with a thin annular detector', J. Electron Microsc. 50 (2001),
147155.
324. J. M. Cowley,
'Electron nanodiffraction methods for measuring medium-range order'. Ultramicroscopy
90 (2002), 197206.
325. V. V. Smirnov and J.
M. Cowley, 'In-line electron- holography with an atomic-focuser source', Phys.
Rev. B65 (2002), 064109.
326. R. C. Mani, S.
Sharma, M. K. Sunkara, J. Gallapalli, R. P. Baldwin, R. Rao,
A. M. Rao and J. M. Cowley, 'Synthesis and electrochemical
characteristics of a nanocomposite diamond electrode', ECS Lett. 5, 6
(2002), E32E35.
327. Carolyn Jones Otten,
Oleg R. Lourie, Min- Feng Yu, John M. Cowley, Mark J. Dyer, Rodney S. Ruoff
and William E. Buhro, 'Crystalline boron nanowires', J. Am. Chem. Soc.
124, 17 (2002), 45644565.
328. J. M. Cowley,
'Ultra-high resolution with off- axis STEM holography', Ultramicroscopy
96, 2 (2003), 163166.
329. J. M. Cowley,
'Off-axis STEM or TEM holography combined with four-dimensional
diffraction-imaging', Micros. Microanal. 10, 1 (2004), 915.
330. J. M. Cowley,
'Applications of electron nanodiffraction', Micron 35, 5 (2004),
345360.
331. C. Quintana, J. M.
Cowley and C. Marhic, 'Electron nanodiffraction and high resolution electron
microscopy studies of the structure and composition of physiological and pathological
ferritin', J. Struct. Biol. 147, 2 (2004), 166178.
332. J. M. Cowley, R. C.
Mani and M. K. Sunkara, 'Structures of carbon nanocrystals', Chem. Mater.
16, 24 (2004), 49054911.
333. M. Loan, J. M.
Cowley and R. Hart, 'Evidence on the structure of synthetic schwertmannite', Am.
Mineral. 89, 11 (2004), 17351742.
334. R.
C. Mani, M. K. Sunkara, R. P. Baldwin, J. G. Gullapalli, J. A. Chaney, G.
Bhimarasetti, J. M. Cowley, A. M. Rao and R. H. Rao, 'Nanocrystalline graphite
for electrochemical sensing', J. Electrochem. Soc. 152, 4 (2005),
E154E159.
2. Papers in conference proceedings (two or more pages)
1. J.
M. Cowley and A. F. Moodie, 'The imaging of crystal lattices and their
imperfections', Proceedings of European Regional Conference on Electron
Microscopy (1961), 199202.
2. J. M. Cowley,
'Electron diffraction from unresolvable defects', Proceedings of Conference on
Electron Diffraction and Crystal Defects, Melbourne 1965, J-5 (1965).
3. J. M. Cowley and
A. P. Pogany, 'Dynamical diffraction from perturbed and disordered crystals', Electron
Microscopy, 1966, Proceedings of 6th International Conference for Electron
Microscopy, Kyoto (1966), 7576.
4. S. Kuwabara, P. S.
Turner and J. M. Cowley, 'Variation of electron diffraction intensities of
BiOC1 lamellar polycrystals with wavelength, crystal thickness filtering',
Electron Microscopy, 1966, Proceedings of the 6th International Congress for
Electron Microscopy, Kyoto (1966), 59.
5. J. M. Cowley and
A. Strojnik, 'A 600kV transmission scanning electron microscope', Electron
Microscopy, 1968, Proceedings of the 4th European Regional Conference on
Electron Microscopy, Rome (1968), 7172.
6. J. M. Cowley and
A. Strojnik, 'A 600kV transmission scanning electron microscope', Scanning
Electron Microscopy 1969, Proceedings of 2nd Annual Scanning Electron
Microscopy Symposium, I. I. T. Research Institute (1969), 1317.
7. J. M. Cowley and
A. Strojnik, 'Design and application of a high-voltage transmission scanning
electron microscope', Proceedings 27th Annual Meeting EMSA (1969), 2728.
8. J. M. Cowley,
'High-voltage scanning electron microscopy', Proceedings of the 28th Annual
EMSA meeting (1970), 67.
9. J. M. Cowley and
G. R. Grinton, 'Calculations of contrast from model biological systems',
Proceedings 28th Annual Meeting EMSA (1970), 30.
10. J. M. Cowley and
Sumio Iijima, 'The interpretation of crystal lattice images', Proceedings
29th Annual Meeting EMSA (1971), 168169.
12. J. M. Cowley, 'New
possibilities for electron diffraction', Proceedings 29th Annual Meeting EMSA
(1971), 172173.
13. J. M. Cowley,
'Analysis of dark-field images of disordered materials', Proceedings 30th
Annual Meeting EMSA (1972), 560561.
14. J. M. Cowley and
Sumio Iijima, 'The interpretation of crystal lattice images', Proceedings
30th Annual Meeting EMSA (1972), 550551.
15. J. R. Sellar and J.
M. Cowley, 'Contrast and resolution in alfresco microscopy and thick
specimens', Proceedings 30th Annual Meeting EMSA (1972), 570571.
16. J. M. Cowley, F. A.
Koch and J. L. Albain, 'Medium energy electron diffraction and scanning
electron microscopy for surface studies', Proceedings of 33rd Conference on
Physical Electronics, Berkeley (1973), 1316.
17. J. M. Cowley, F. A.
Koch and J. L. Albain, 'An experimental system combining medium energy electron
diffraction and scanning electron microscopy', 31st Annual Proceedings EMSA
(1973), 136137.
18. W. H. Massover and
J. M. Cowley, 'High resolution lattice images of ferritin core crystallites',
in 31st Annual Proceedings EMSA (1973), 598599.
19. J. M. Cowley, 'A
comparison of scanning and fixed beam high voltage electron microscopy', 31st
Annual Proceedings EMSA (1973), 67.
20. J. M. Cowley,
'Contrast in high resolution bright-field and dark-field images of thin
specimens', 31st Annual Proceedings EMSA (1973), 222223.
21. J. M. Cowley, 'High
voltage SEM: Contrast theory and applications', in High Voltage Electron Microscopy, ed. P. R. Swann, C. J. Humphreys and M. J. Goringe
(Academic Press, London and New York, 1974), pp. 7684.
22. J. M. Cowley, 'The
interpretation of electron diffraction patterns of faulted structures', in 32nd
Annual Proceedings EMSA (1974), 342343.
23. J. L. Albain, J. M.
Cowley, P. E. Hψjlund Nielsen, F. A. Koch and H. Shuman, 'Surface studies with
medium energy electron diffraction (MEED)', 32nd Annual Proceedings EMSA
(1974), 414415.
24. H. Shuman and J. M.
Cowley, 'Surface diffraction imaging of lattice defects', 32nd Annual
Proceedings EMSA (1974), 344345.
25. J. M. Cowley,
'Scanning transmission electron microscopy of thick and crystalline
specimens', in Electron Microscopy/1974, Vol. I, pp. 1819
(Proceedings of Eighth International Conference on Electron Microscopy,
Canberra, 1974).
26. J. L. Albain, J. M.
Cowley, P. E. Hψjlund Nielsen, F. A. Koch and H. Shuman, 'Reflection electron
microscopy using diffracted beams', in Electron Microscopy/1974,
Vol. I, pp. 6263 (1974).
27. H. T. Pearce-Pearcy
and J. M. Cowley, 'Application of energy analysis to STEM', in Electron Microscopy/1974, Vol. I, pp. 394395 (1974).
28. J. M. Cowley, 'A
comparison of scanning and fixed beam high voltage electron microscopy', in Electron Microscopy and Microbeam Analyses, ed. B. M. Siegel
and D. R. Beaman (John Wiley & Sons, New York, 1975), pp. 1728.
29. J. M. Cowley,
'Contrast in high resolution bright field and dark field images of thin
specimens', in Electron Microscopy and Microbeam Analyses,
ed. B. M. Siegel and D. R. Beaman (John Wiley & Sons, New York, 1975),
pp. 315.
30. J. D. Landry, P. E.
Hψjlund Nielsen, G. G. Hembree and J. M. Cowley, 'Medium energy
electron study of surface structures formed upon oxidation of copper', 33rd
Annual Proceedings EMSA, ed. G. W. Bailey (1975), 6667.
31. P. E. Hψjlund
Nielsen and J. M. Cowley, 'Reflection electron microscopy', 33rd Annual
Proceedings EMSA, ed. G. W. Bailey (1975), 122123.
32. J. M. Cowley,
'Potentialities and problems of high resolution', in High Voltage Electron Microscopy/1975, Fourth International Conference, Toulouse (1975), 129134.
34. J. M. Cowley,
'Intensity distributions in high resolution images of thin crystals', Microscopical
Society of Canada, Vol. III (1976), 1415.
35. J. M. Cowley,
'Image Contrast for Dark-field STEM', 34th Annual Proceedings EMSA, ed. G. W.
Bailey (1976), 466467.
36. J. M. Cowley and
Bing K. Jap, 'The use of diffraction pattern information in STEM', 34th Annual
Proceedings EMSA, ed. G. W. Bailey (1976), 460461.
37. G. G. Hembree, M.
A. Otooni and J. M. Cowley, 'Studies of oxide formation on copper
thin films by reflection electron microscopy', 35th Annual Proceedings EMSA
(1977), 316317.
38. P. M. Fields and J.
M. Cowley, 'Computer simulation of the imaging of atomic defects in metals',
35th Annual Proceedings EMSA (1977), 1415.
39. J. M. Cowley, 'High
voltage STEM contrast theory and applications', in High Voltage Electron Microscopy, 1977, Proceedings of the 5th
International Conference on HVEM, Kyoto (1977), 914.
40. J. M. Cowley, 'The
imaging of crystal structures and crystal defects', in Electron Microscopy 1978, Vol. III: State of the Art Symposia, ed. J. M. Sturgess (Microscopical Society of Canada, Toronto,
1978), pp. 207217.
41. G. G. Hembree, J.
M. Cowley and M. A. Otooni, 'A RMEED and SEM investigation of metal
oxidation phenomena', Electron Microscopy 1978, Vol. I, ed. J. M. Sturgess (Microscopical Society of
Canada, Toronto, 1978), pp. 444445.
42. J. M. Cowley and
Andrew Y. Au, 'Bright-field image contrast and resolution in STEM and CTEM', Electron Microscopy 1978, Vol. I, ed. J. M. Sturgess
(Microscopical Society of Canada, Toronto, 1978), pp. 172173.
43. J. M. Cowley and P.
M. Fields, 'Imaging and diffraction from localized defects and disorder in
crystals', Electron Microscopy 1978, Vol. I,
ed. J. M. Sturgess Microscopical Society of Canada, Toronto, 1978), pp.
240241.
44. Fumio Watari and J.
M. Cowley, 'Study of oxidation on the surface of chromium by STEM', 37th Annual
Proceedings EMSA (Claitor's Publication Division, Baton Rouge, LA, 1979),
472473.
45. J. M. Cowley, 'STEM
imaging with an optical analyzer detection system', 37th Annual Proceedings
EMSA, ed. G. W. Bailey (Claitor's Publication Division, Baton Rouge, LA, 1979),
472473.
46. J. M. Cowley,
'Application of a STEM instrument to the study of crystals', in Electron Microscopy and Analysis 1979, ed. T. Mulvey
(Institute of Physics, London, 1980), pp. 239355.
47. J. M. Cowley, P.
Goodman, P. S. Turner and M. Disko, 'Interference effects in shadow image
electron microscopy (STEM) and in STEM and CTEM of surfaces', 38th Annual
Proccedings EMSA, ed. G. W. Bailey (Claitors Publication Division, Baton Rouge,
LA, 1980), 164165.
48. Fumio Watari and J.
M. Cowley, 'STEM and ELS observation of early oxide formation on the surface of
Cr thin films', 38th Annual Proceedings EMSA, ed. G.W. Bailey (Claitor's
Publication Division, Baton Rouge, LA, 1980), 412413.
49. P. S. Turner and J.
M. Cowley, 'Reflection and refraction imaging of oxide surfaces in TEM and
STEM', Electron Microscopy 1980, ed. P. Brederoo and G.
Boom (Seventh European Congress on Electron Microscopy Foundation, Leiden,
1980), Vol. 1, pp. 390391.
50. J. M. Cowley and
Fumio Watari, 'Application of Microdiffraction with a STEM instrument', in Electron Microscopy 1980, ed. P. Brederoo and G. Boom (Seventh
European Congress on Electron Microscopy Foundation, Leiden, 1980), Vol. 3,
pp. 176177.
51. J. M. Cowley,
'Imaging and analysis of surfaces using diffracted electrons', 39th Annual
Meeting EMSA, ed. G. W. Bailey (Claitor's Publication Division, Baton Rouge,
LA, 1981), 211215.
52. J. M. Cowley,
'Rapid recording of microdiffraction with a STEM instrument', 39th Annual Proceedings EMSA,
ed. G. W. Bailey (Claitor's Publication Division, Baton Rouge, LA, 1981),
348349.
53. J. C. H. Spence and
J. M. Cowley, 'An X-ray laser at electron microscope voltages?', 39th Annual
Proceedings EMSA, ed. G. W. Bailey (Claitor's Publication Division, Baton
Rouge, LA, 1981), 380381.
54. I. Y. T. Chan and
J. M. Cowley, 'Microdiffraction study of short-range ordering in LiFeO2', 39th
Annual Proceedings EMSA, ed. G. W. Bailey (Claitor's Publication Division,
Baton Rouge, LA, 1981), 350351.
55. F. Watari, J. H.
Butler, A. Higgs and J. M. Cowley, 'Application of STEM-Digital system for ELS
mapping', Electron Microscopy 1982, ed. Congress
Organizing Committee, Deutsche Gesellschaft fόr Elektronenmikroskopie eV,
Frankfurt/Main, 1982), Vol. 1, pp. 593594.
56. J. M. Cowley, Jing
Zhu and Z. C. Kang, 'Microdiffraction studies of planar defects and surface
reactions of crystals', Electron Microscopy 1982, ed.
Congress Organizing Committee, Deutsche Gesellschaft fόr Elektronenmikroskopie
eV, Frankfurt/Main, 1982), Vol. 1, pp. 633634.
57. H. Q. Ye and J. M.
Cowley, 'High resolution imaging of Mo5O14 and Mo17O47', Electron Microscopy 1982, ed. Congress Organizing Committee, Deutsche Gesellschaft fόr
Elektronenmikroskopie eV, Frankfurt/Main, 1982), Vol. 2, pp. 910.
58. J. M. Cowley,
'Surface channelling effects in microdiffraction, STEM and EELS', Electron Microscopy 1982, ed. Congress Organizing Committee, Deutsche
Gesellschaft fόr Elektronenmikroskopie eV, Frankfurt/Main, 1982), Vol. 2, pp.
283284.
59. R. W. Carpenter, I.
Y. T. Chan and J. M. Cowley, 'CBED shadow images and Cs-aberration
measurement', 39th Annual Proceedings EMSA, ed. G. W. Bailey (Claitor's
Publication Division, Baton Rouge, LA, 1981), 5657.
60. J. M. Cowley and W.
B. Monosmith, 'STEM studies of small metal particles', Proceedings of the 41st
Annual Meeting EMSA, ed. G. W. Bailey (San Francisco Press, San Francisco,
1983), pp. 332333.
61. J. M. Cowley, W. B.
Monosmith and M. M. Disko, 'Pattern recognition techniques applied to
microdiffraction patterns', Proceedings of the 41st Annual Meeting EMSA, ed.
G. W. Bailey (San Francisco Press, San Francisco, 1983), 302303.
62. C.-S. Tan and J. M.
Cowley, 'A micro-refraction study of the potential field outside a gold
crystal', Proceedings of the 41st Annual Meeting EMSA, ed. G. W. Bailey (San
Francisco Press, San Francisco, 1983), 300301.
63. C. E. Warble and J.
M. Cowley, 'Pd/MgO Reaction Study', Proceedings of the 41st Annual Meeting
EMSA, ed. G. W. Bailey (San Francisco Press, San Francisco, 1983), 330331.
64. J. M. Cowley,
'Reflection electron microscopy and diffraction from crystal surfaces', Proceedings
of the Materials Research Society Symposium, Vol. 31 (1984), 177188.
65. Nobuo Tanaka,
Ken-ichi Ohshima, Jimpei Harada and J. M. Cowley, 'High resolution observations
of short-range ordering in disordered Au4Mn alloys', Proceedings of the 42nd
Annual Meeting EMSA, ed. G.W. Bailey (San Francisco Press, San Francisco,
1984), 426427.
66. Nobuo Tanaka and J.
M. Cowley, 'High resolution electron microscopy of disordered LiFeO2',
Proceedings of the 42nd Annual Meeting EMSA, ed. G.W. Bailey (San Francisco
Press, San Francisco, 1984), 430431.
67. J. M. Cowley and Z.
L. Wang, 'The deflection of electron beams traversing a crystal face',
Proceedings of the 43rd Annual Meeting EMSA, ed. G.W. Bailey (San Francisco
Press, San Francisco, 1985), 6263.
68. J. A. Lin and J. M.
Cowley, 'In-line electron holography in a STEM instrument', Proceedings of the
43rd Annual Meeting EMSA, ed. G.W. Bailey (San Francisco Press, San Francisco,
1985), 136137.
69. G. Y. Fan and J. M.
Cowley, 'Auto-correlation analysis of high resolution electron micrographs of
near-amorphous thin films', Proceedings of the 43rd Annual Meeting EMSA, ed.
G.W. Bailey (San Francisco Press, San Francisco, 1985), 6061.
70. J. M. Cowley, 'A
new detector system for the HB5 STEM instrument', Proceedings of the 43rd
Annual Meeting EMSA, ed. G. W. Bailey (San Francisco Press, San Francisco,
1985), 134135.
71. S. Y. Zhang and J.
M. Cowley, 'The observation of MgOAl interface by HREM and microdiffraction',
Proceedings of the 43rd Annual Meeting EMSA, ed. G.W. Bailey (San Francisco
Press, San Francisco, 1985), 240241.
72. J. M. Cowley, R.
Glaisher, J. A. Lin and H.‑J. Ou, 'Imaging and diffraction modes in
scanning transmission electron microscopy', Proceedings of the 44th Annual
Meeting EMSA (1986), 684687.
73. G.-Y. Fan and J. M.
Cowley, 'Soft-ware pattern recognition applied to microdiffraction patterns from a STEM
instrument', Proceedings of the 44th Annual Meeting EMSA (1986), 694695.
74. G.-Y. Fan and J. M.
Cowley, 'Simulations of high resolution images of amorphous silicon films',
Proceedings of the 44th Annual Meeting EMSA (1986), 544545.
75. L. M. Peng and J.
M. Cowley, 'A multislice approach to the RHEED and REM simulation',
Proceedings of the 44th Annual Meeting EMSA (1986), 380381.
76. J. M. Cowley, 'High
resolution imaging and diffraction studies of crystal surfaces', Electron
Microscopy 1 (1986), 38.
77. J. M. Cowley,
'Scanning electron microscopy and electron diffraction', Electron Microscopy
1 (1986), 7174.
78. H.-J. Ou and J. M.
Cowley, 'Investigation of electron-beam induced nucleation by scanning
reflection electron microscopy', Electron Microscopy 2 (1986),
13611362.
78a. T. Tanji, H.
Masaoka, K. Yada and J. M. Cowley, 'Interactions of electron beams
with surfaces of small MgO crystals', Electron Microscopy 2
(1986), 13531354.
79. L.-M. Peng, J. M.
Cowley and Tung Hsu, 'The surface step: Its strain field and REM image contrast
splitting', Proceedings of the 45th Annual Meeting EMSA, ed.
G. W. Bailey (San Francisco Press, San Francisco, 1987), 3435.
80. L.-M. Peng, J. M.
Cowley and Tung Hsu, 'Effects of surface stress relaxation on reflection
electron microscopy images of normal emerging edge dislocations', Proceedings
of the 45th Annual Meeting EMSA, ed. G. W. Bailey (San Francisco
Press, San Francisco, 1987), 3637.
81. J. Liu and J. M.
Cowley, 'Electron beam radiation effects on NiO crystals', Proceedings of the
45th Annual Meeting EMSA, ed. G. W. Bailey (San Francisco Press, San
Francisco, 1987), 176177.
82. M. Pan, J. M.
Cowley, I. Y. Chan and R. Garcia, 'Structure studies of supported metal
catalyst particles by microdiffraction technique', Proceedings of the 45th
Annual Meeting EMSA, ed. G. W. Bailey (San Francisco Press, San Francisco,
1987), 202203.
83. Z.-L. Wang and J.
M. Cowley, 'Atomic inner shell excitations with EELS in REM: Pt and Au M4.5
edge shapes modifications in REM', Proceedings of the 45th Annual Meeting
EMSA, ed. G. W. Bailey (San Francisco Press, San Francisco, 1987), 402403.
84. Z.-L. Wang and J.
M. Cowley, 'EELS characterization of bulk crystal surfaces in REM: Surfaces
microanalysis and surface channelling effect', Proceedings of the 45th Annual
Meeting EMSA, ed. G. W. Bailey (San Francisco Press, San Francisco, 1987),
398399.
85. Z.-L. Wang and J.
M. Cowley, 'The dependences of the surface plasmon frequencies on the
supported metal particle sizes and shapes', Proceedings of the 45th Annual
Meeting EMSA, ed. G. W. Bailey (San Francisco Press, San Francisco, 1987),
130131.
86. Z.-L. Wang and J.
M. Cowley, 'Generation of surface plasmons in a supported metal particle with
an external electron beam. I. Quantum theory', Proceedings of the 45th Annual
Meeting EMSA, ed. G. W. Bailey (San Francisco Press, San Francisco, 1987),
404405.
87. Z.-L. Wang and J.
M. Cowley, 'Generation of surface plasmons in a supported metal particle with
an external electron beam. II. Classical energy loss theory', Proceedings of
the 45th Annual Meeting EMSA, ed. G. W. Bailey (San Francisco Press, San
Francisco, 1987), 406407.
88. P. R. Swann, J. S.
Jones, O. L. Krivanek, D. J. Smith, J. A. Venables and J. M. Cowley,
'UHV conversion of a 300 kV high-resolution electron microscope', Proceedings
of the 45th Annual Meeting EMSA, ed. G. W. Bailey (San Francisco
Press, San Francisco, 1987), 136137.
89. J. A. Venables, J.
M. Cowley and H. S. von Harrach, 'A field-emission STEM for
surface studies', Inst. Phys. Conf. Ser. No. 90 (IOP Publishing, London, 1987),
Chapter 4, 8184.
90. J. Liu and J. M.
Cowley, 'SEM and microdiffraction study of the reduction of metal oxides in a
STEM instrument', Proceedings of the 46th Annual Meeting EMSA, ed.
G. W. Bailey (San Francisco Press, San Francisco, 1988), 516517.
91. J. Liu and J. M.
Cowley, 'Ultra-high resolution SEM in a STEM instrument', Proceedings of the
46th Annual Meeting EMSA, ed. G. W. Bailey (San Francisco Press, San Francisco,
1988), 182183.
92. J. M. Cowley and P.
A. Crozier, 'Surface resonance channelling in scanning reflection electron
microscopy', Proceedings of the 46th Annual Meeting EMSA, ed.
G. W. Bailey (San Francisco Press, San Francisco, 1988), 692693.
93. L.-M. Peng, J. M.
Cowley and Tung Hsu, 'Identification of dislocations on crystal surfaces',
Proceedings of the 46th Annual Meeting EMSA, ed. G. W. Bailey (San Francisco
Press, San Francisco, 1988), 688689.
94. L.-M. Peng and J.
M. Cowley, 'Reflection monolayer scattering and RHEED diffraction conditions', Proceedings
of the 46th Annual Meeting EMSA, ed. G. W. Bailey (San Francisco Press, San
Francisco, 1988), 962963.
95. H.-J. Ou and J. M.
Cowley, 'High resolution STEM imaging study on high Tc superconductor
YBa2Cu3O7-x', Proceedings of the 46th Annual Meeting EMSA, ed. G. W. Bailey
(San Francisco Press, San Francisco, 1988), 680681.
96. M. Pan and J. M.
Cowley, 'The effects of surface absorbed monolayer on electron microdiffraction
patterns', Proceedings of the 46th Annual Meeting EMSA, ed. G. W. Bailey (San
Francisco Press, San Francisco, 1988), 3233.
97. N. Yao and J. M.
Cowley, 'REM and RHEED investigation of the epitaxy of evaporated gold film on
a GaAs (110) surface', Proceedings of the 46th Annual Meeting EMSA, ed. G. W.
Bailey (San Francisco Press, San Francisco, 1988), 690691.
98. N. Yao and J. M.
Cowley, 'Characterization of double contours and twin images in REM',
Proceedings of the 46th Annual Meeting EMSA, ed. G. W. Bailey (San Francisco
Press, San Francisco, 1988), 686687.
99. M.
Gajdardziska-Josifovska and J. M. Cowley, 'A novel technique for studying interface
abruptness in a STEM', Proceedings of the 47th Annual Meeting EMSA, ed.
G. W. Bailey (San Francisco Press, San Francisco, 1989), 524525.
100. M.
Gajdardziska-Josifovska and J. M. Cowley, 'Geometrical explanation of parabolas
and resonance in electron diffraction', Proceedings of the 47th Annual Meeting
EMSA, ed. G. W. Bailey (San Francisco Press, San Francisco, 1989),
498499.
101. H.-J. Ou, A. A.
Higgs, P. R. Perkes and J. M. Cowley, 'High spatial resolution microanalysis
on the (200) nanodiffraction intensity to determine Al concentration of
AlGaAs-GaAs MQWS', Proceedings of the 47th Annual Meeting EMSA, ed.
G. W. Bailey (San Francisco Press, San Francisco, 1989), 232233.
102. G. C. Ndubuisi, J.
Liu and J. M. Cowley, 'Annealing effects on the sapphire (0001) surface',
Proceedings of the 47th Annual Meeting EMSA, ed. G. W. Bailey (San Francisco
Press, San Francisco, 1989), 544545.
103. J. Liu and J. M.
Cowley, 'SREM imaging of copper (110) vicinal surfaces', Proceedings of the
47th Annual Meeting EMSA, ed. G. W. Bailey (San Francisco Press, San
Francisco, 1989), 542543.
104. M. Pan, R. Garcia,
D. J. Smith, J. M. Cowley and G. A. Cifredo, 'Electron microscopy study of
metal-support interaction in Rh/CeO2 catalysts', Proceedings of the
47th Annual Meeting EMSA, ed. G. W. Bailey (San Francisco Press, San Francisco,
1989), 478479.
105. Nan Yao and J. M.
Cowley, 'Acceleration voltage effect on electron surface channelling',
Proceedings of the 47th Annual Meeting EMSA, ed. G. W. Bailey (San Francisco
Press, San Francisco, 1989), 530531.
106. Nan Yao and J. M.
Cowley, 'Convergence of the incident beam in reflection electron microscopy',
Proceedings of the 47th Annual Meeting EMSA, ed. G. W. Bailey (San Francisco
Press, San Francisco, 1989), 378379.
107. J. Liu and J. M.
Cowley, 'Valence electron energy loss spectroscopy in reflection geometry',
Proceedings of the 47th Annual Meeting EMSA, ed. G. W. Bailey (San Francisco
Press, San Francisco, 1989), 146147.
108. J. Liu and J. M.
Cowley, 'Scanning reflection electron imaging of crystal surfaces', Proceedings
of the 47th Annual Meeting EMSA, ed. G. W. Bailey (San Francisco Press, San
Francisco, 1989), 538539.
109. P. A. Crozier, J.
Liu and J. M. Cowley, 'Secondary electron imaging of MoO3 reduction
in a UHV STEM', Proceedings of the 47th Annual Meeting EMSA, ed. G. W. Bailey
(San Francisco Press, San Francisco, 1989), 8687.
110. P. A. Crozier, J.
Liu and J. M. Cowley, 'Microdiffraction from very small crystals', Proceedings
of the 47th Annual Meeting EMSA, ed. G. W. Bailey (San Francisco Press, San
Francisco, 1989), 520521.
111. H.-J. Ou, R. W.
Glaisher, J. M. Cowley and H. Morkoc, 'Using the (200) thickness contour
to measure the absolute Al concentration of AlxGa1-xAs-GaAs MQWS structures',
Proceedings of the Microbeam Analyses Society Meeting (San Francisco Press, San
Francisco, 1989), 480482.
112. N. Tanaka, K.
Mihama, M. Skiff, R. Graham and J. M. Cowley, 'EELS of nano-crystals embedded
in MgO', Proceedings of the Materials Research Society 139 (1989), 3843.
113. H.-J. Ou, A. A.
Higgs and J. M. Cowley, 'High resolution STEM images and nanodiffraction
patterns on high-Tc superconductor YBa2Cu3O7-x', Proceedings of the Materials
Research Society 139 (1989), 223228.
114. J. M. Cowley, 'High
resolution scanning electron microscopy of surfaces', Proceedings of the XIIth
International Congress for Electron Microscopy, ed. L. D. Peachey and
D. B. Williams (San Francisco Press, San Francisco, 1990), Vol. 1,
296297.
115. M. Gajdardziska-Josifovska,
P. A. Crozier and J. M. Cowley, 'The influence of annealing on the Topography
of (100) and (111) surfaces of MgO', Proceedings of the XIIth International
Congress for Electron Microscopy, ed. L. D. Peachey and D. B. Williams (San
Francisco Press, San Francisco, 1990), Vol. 4, 232233.
116. G. C. Ndubuisi, J.
Liu and J. M. Cowley, 'REM observation of the prismatic faces of sapphire',
Proceedings of the XIIth International Congress for Electron Microscopy, ed.
L. D. Peachey and D. B. Williams (San Francisco Press, San Francisco, 1990),
Vol. 1, 330331.
117. P. A. Crozier, M.
Gajdardziska-Josifovska and J. M. Cowley, 'Observation of reconstruction on
(111) surfaces of MgO', Proceedings of the XIIth International Congress for
Electron Microscopy, ed. L. D. Peachey and D. B. Williams (San Francisco Press,
San Francisco, 1990), Vol. 4, 280281.
118. Nan Yao and J. M.
Cowley, 'Characterization of surface resonance conditions for surface imaging',
Proceedings of the XIIth International Con |